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1.
Pioneer Venus ultraviolet spectra from the first 5 years of operation show a decline (by more than a factor of 10) in sulfur dioxide abundance at the cloud tops and in the amount of submicron haze above the clouds. At the time of the Pioneer Venus encounter, the values for both parameters greatly exceeded earlier upper limits. However, Venus had a similar appearance in the late 1950's, implying the episodic injection of sulfur dioxide possibly caused by episodic volcanism. The amount of haze in the Venus middle atmosphere is about ten times that found in Earth's stratosphere after the most recent major volcanic eruptions, and the thermal energy required for this injection on Venus is greater by about an order of magnitude than the largest of these recent Earth eruptions and about as large as the Krakatoa eruption of 1883. The episodic behavior of sulfur dioxide implies that steady-state models of the chemistry and dynamics of cloud-top regions may be of limited use.  相似文献   

2.
Gas emissions and the eruptions of mount st. Helens through 1982   总被引:3,自引:0,他引:3  
The monitoring of gas emissions from Mount St. Helens includes daily airborne measurements of sulfur dioxide in the volcanic plume and monthly sampling of gases from crater fumaroles. The composition of the fumarolic gases has changed slightly since 1980: the water content increased from 90 to 98 percent, and the carbon dioxide concentrations decreased from about 10 to 1 percent. The emission rates of sulfur dioxide and carbon dioxide were at their peak during July and August 1980, decreased rapidly in late 1980, and have remained low and decreased slightly through 1981 and 1982. These patterns suggest steady outgassing of a single batch of magma (with a volume of not less than 0.3 cubic kilometer) to which no significant new magma has been added since mid-1980. The gas data were useful in predicting eruptions in August 1980 and June 1981.  相似文献   

3.
The Nabro stratovolcano in Eritrea, northeastern Africa, erupted on 13 June 2011, injecting approximately 1.3 teragrams of sulfur dioxide (SO(2)) to altitudes of 9 to 14 kilometers in the upper troposphere, which resulted in a large aerosol enhancement in the stratosphere. The SO(2) was lofted into the lower stratosphere by deep convection and the circulation associated with the Asian summer monsoon while gradually converting to sulfate aerosol. This demonstrates that to affect climate, volcanic eruptions need not be strong enough to inject sulfur directly to the stratosphere.  相似文献   

4.
The observed mass-independent sulfur isotopic composition (Delta33S) of volcanic sulfate from the Agung (March 1963) and Pinatubo (June 1991) eruptions recorded in the Antarctic snow provides a mechanism for documenting stratospheric events. The sign of Delta33S changes over time from an initial positive component to a negative value. Delta33S is created during photochemical oxidation of sulfur dioxide to sulfuric acid on a monthly time scale, which indicates a fast process. The reproducibility of the results reveals that Delta33S is a reliable tracer to chemically identify atmospheric processes involved during stratospheric volcanism.  相似文献   

5.
On 9 April 1984, commercial airlines enroute from Tokyo, Japan, to Anchorage, Alaska, reported an unusual mushroom-shaped cloud at about 38.5 degrees N, 146.0 degrees E. On 8 and 9 April the intensity of volcanism from Kaitoku Seamount (26.0 degrees N, 140.8 degrees E), as indicated by T-phase recordings on an array of ocean bottom hydrophones, reached a maximum level and then declined rapidly. An examination was made of the possible relation of the cloud to eruptions of Kaitoku through an analysis of pilot depositions, satellite photos, wind charts, signal strengths and spectra of known man-made underwater explosions, as well as ascent rates of volcanic plumes and cumulonimbus clouds.  相似文献   

6.
The first extensive measurements by remote-sensing correlation spectrometry of the sulfur dioxide emitted by volcanic plumes indicate that on the order of 10(3) metric tons of sulfur dioxide gas enter the atmosphere daily from Central American volcanoes. Extrapolation gives a minimum estimate of the annual amount of sulfur dioxide emitted from the world's volcanoes of about 10(7) metric tons.  相似文献   

7.
Ash from the massive 18 May 1980 eruption of Mount St. Helens readily gave off large amounts of carbonyl sulfide and carbon disulfide gases at room temperature. These findings suggest that the sulfur that enhances the Junge sulfate layer in the stratosphere after volcanic eruptions could be carried directly to the upper atmosphere as carbonyl sulfide and carbon disulfide adsorbed on ash particles from major volcanic eruptions.  相似文献   

8.
Several photometric measurements of Venus made from the Pioneer Venus orbiter and probes indicate that solar near-ultraviolet radiation is being absorbed throughout much of the main cloud region, but little above the clouds or within the first one or two optical depths. Radiative transfer calculations were carried out to simulate both Pioneer Venus and ground-based data for a number of proposed cloud compositions. This comparison rules out models invoking nitrogen dioxide, meteoritic material, and volatile metals as the source of the ultraviolet absorption. Models involving either small ( approximately 1 micrometer) or large ( approximately 10 micrometers) sulfur particles have some serious difficulties, while ones invoking sulfur dioxide gas appear to be promising.  相似文献   

9.
During the steady-state period of activity of La Soufriere Volcano in 1979, the mass emissions of sulfur dioxide into the troposphere amounted to a mean value of 339 +/- 126 metric tons per day. This value is similar to the sulfur dioxide emissions of other Central American volcanoes but less than those measured at Mount Etna, an exceptionally strong volcanic source of sulfur dioxide.  相似文献   

10.
Hanel R  Conrath B 《Science (New York, N.Y.)》1969,165(3899):1258-1260
A Michelson interferometer spectrometer carried aboard the Nimbus 3 satellite, launched 14 April 1969, measured the spectrum between 400 and 2000 wave numbers with a resolution of 5 wave numbers. High-quality spectra have been obtained on a global scale, and preliminary results indicate that the absorption bands of carbon dioxide, water vapor, and ozone can be used to obtain vertical distributions of temperature, water vapor, and ozone.  相似文献   

11.
Spectroscopic observations of the total column amount of hydrogen chloride above an altitude of 12 kilometers in the latitude range 20 degrees to 40 degrees N have been made both before and 3 to 6 months after the eruptions of El Chichón Volcano in March and April 1982. In the region of the cloud of volcanic aerosols, the hydrogen chloride total column after the eruptions increased by approximately 40 percent, even after allowance is made for the global secular increase in hydrogen chloride of 5 percent per year. The column amounts of hydrogen fluoride show no such increase.  相似文献   

12.
In this report the fluxes measured by the solar flux radiometer (LSFR) of the Pioneer Venus large probe are compared with calculations for model atmospheres. If the large particles of the middle and lower clouds are assumed to be sulfur, strong, short-wavelength absorption results in a net flux profile significantly different from the LSFR net flux measurements. Models in which the smallest particles are assumed to be sulfur gave flux profiles consistent with the measurements if an additional source of absorption is included in the upper cloud. The narrowband data from 0.590 to 0.665 micrometer indicate an absorption optical depth of about 0.05 below the cloud bottom. The broadband data imply that either this absorption extends over a considerable wavelength interval (as might be the case for dust) or that a very strong absorption band lies on one side of the narrowband filter (as suggested by early Venera 11 and Venera 12 reports). Thermal balance calculations based on the measured visible fluxes indicate high surface temperature for reasonable assumptions of cloud opacity and water vapor abundance. The lapse rate becomes convective within the middle cloud. For water mixing ratios of 2.0 x 10(-4) below the clouds we find a subadiabatic region extending from the cloud bottom to altitudes near 35 kilometers.  相似文献   

13.
Sulfur dioxide (SO(2)) released by the explosive eruption of Mount Pinatubo on 15 June 1991 had an impact on climate and stratospheric ozone. The total mass of SO(2) released was much greater than the amount dissolved in the magma before the eruption, and thus an additional source for the excess SO(2) is required. Infrared spectroscopic analyses of dissolved water and carbon dioxide in glass inclusions from quartz phenocrysts demonstrate that before eruption the magma contained a separate, SO(2)-bearing vapor phase. Data for gas emissions from other volcanoes in subduction-related arcs suggest that preeruptive magmatic vapor is a major source of the SO(2) that is released during many volcanic eruptions.  相似文献   

14.
High rates of volcanic and tectonic activities are inferred from Venus's high surface temperature. The effects of volcanic effluents, gas and dust, on obscuration in the atmosphere are considered. The optical extinction due to particulate matter is estimated from assumed distributions as to particle size and altitude. As few as ten explosive eruptions per annum would cause significant absorption and scattering of visible light.  相似文献   

15.
Initial examination of data from the neutral mass spectrometer on the Pioneer Venus sounder probe indicates that the abundances of argon-36, argon-38, and neon-20 in the Venus atmosphere are much higher than those of the corresponding gases in Earth's atmosphere, although the abundance of radiogenic argon-40 is apparently similar for both planets. The lower atmosphere of Venus includes significant concentrations of various gaseous sulfur compounds. The inlet leak to the mass spectrometer was temporarily blocked by an apparently liquid component of the Venus clouds during passage through the dense cloud layer. Analysis of gases released during the evaporation of the droplets shows the presence of water vapor to some compound or compounds of sulfur.  相似文献   

16.
The first gas chromatographic analysis of the lower atmosphere of Venus is reported. Three atmospheric samples were analyzed. The third of these samples showed carbon dioxide (96.4 percent), molecular nitrogen (3.41 percent), water vapor (0.135 percent), molecular oxygen [69.3 parts per million (ppm)], argon (18.6 ppm), neon (4.31 ppm), and sulfuir dioxide (186 ppm). The amounts of water vapor and sulfur dioxide detected are roughly compatible with the requirements of greenhouse models of the high surface temperature of Venus. The large positive gradient of sulfur dioxide, molecular oxygen, and water vapor from the clould tops to their bottoms, as implied by Earth-based observations and these resuilts, gives added support for the presence of major quantities of aqueous sulfuric acid in the clouds. A comparison of the inventory of inert gases found in the atmospheres of Venus, Earth, and Mars suggests that these components are due to outgassing from the planetary interiors.  相似文献   

17.
Hawaiian plants exposed to volcanic sulfur dioxide showed interspecific differences in leaf injury that are related to sulfur dioxide-induced changes in stomatal condutance. Species with leaves that did not close stomata developed either chlorosis or necrosis, whereas leaves of Metrosideros collina closed stomata and showed no visual symptoms of sulfur dioxide stress.  相似文献   

18.
Infrared spectral images of Jupiter's volcanic moon Io, acquired during the October and November 1999 and February 2000 flybys of the Galileo spacecraft, were used to study the thermal structure and sulfur dioxide distribution of active volcanoes. Loki Patera, the solar system's most powerful known volcano, exhibits large expanses of dark, cooling lava on its caldera floor. Prometheus, the site of long-lived plume activity, has two major areas of thermal emission, which support ideas of plume migration. Sulfur dioxide deposits were mapped at local scales and show a more complex relationship to surface colors than previously thought, indicating the presence of other sulfur compounds.  相似文献   

19.
Sulfate concentrations from continuous biyearly sampling of the GISP2 Greenland ice core provide a record of potential climate-forcing volcanism since 7000 B.C. Although 85 percent of the events recorded over the last 2000 years were matched to documented volcanic eruptions, only about 30 percent of the events from 1 to 7000 B.C. were matched to such events. Several historic eruptions may have been greater sulfur producers than previously thought. There are three times as many events from 5000 to 7000 B.C. as over the last two millennia with sulfate deposition equal to or up to five times that of the largest known historical eruptions. This increased volcanism in the early Holocene may have contributed to climatic cooling.  相似文献   

20.
At least four active geyser-like eruptions were discovered in Voyager 2 images of Triton, Neptune's large satellite. The two best documented eruptions occur as columns of dark material rising to an altitude of about 8 kilometers where dark clouds of material are left suspended to drift downwind over 100 kilometers. The radii of the rising columns appear to be in the range of several tens of meters to a kilometer. One model for the mechanism to drive the plumes involves heating of nitrogen ice in a subsurface greenhouse environment; nitrogen gas pressurized by the solar heating explosively vents to the surface carrying clouds of ice and dark partides into the atmosphere. A temperature increase of less than 4 kelvins above the ambient surface value of 38 +/- 3 kelvins is more than adequate to drive the plumes to an 8-kilometer altitude. The mass flux in the trailing clouds is estimated to consist of up to 10 kilograms of fine dark particles per second or twice as much nitrogen ice and perhaps several hundred or more kilograms of nitrogen gas per second. Each eruption may last a year or more, during which on the order of a tenth of a cubic kilometer of ice is sublimed.  相似文献   

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