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1.
The mineralogies of ‘Tirs’ (Typic Pelloxererts), and ‘Debs’ (Typic Haploxerolls and Typic Xerochrepts) soils of the Gharb plain in north-western Morocco are investigated, with special attention given to the determination of the nature of the smectitic phase using the lithium test (Li test) and the alkylammonium method. The sand and silt mineralogy of Tirs soils is dominated by quartz with small amounts of feldspars and kaolinite. The sand and silt fractions of Dehs soils also contain significant amounts of mica, chlorite, and interstratified phyllosilicates. The clay minerals of Tirs soils are predominantly a high-charge smectite. The estimated interlayer charge for this phase is 0.61 mol(c)/O10(OH)2 and the fraction of tetrahedral charge varies from 38 to 44%. Although the percentage tetrahedral charge is less than 50%, the smectitic phase behaves as beidellite with the Li test. Dehs clays are more heterogeneous, consisting of smectite, vermiculite, illite, kaolinite, chlorite, and interstratified illite/smectite and illite/vermiculite. The Li test and the alkylammonium method demonstrate that a high-charge smectite or vermiculite is interstratified with illite. A low-charge montmorillonite is also present both in Tirs and in Dehs soils. The high-charge beidellitic phase is believed to be a transformation product of mica, whilst the low charge montmorillonite is thought to be inherited from the parent material.  相似文献   

2.
Accurate estimation of the available potassium (K+) supplied by calcareous soils in arid and semi‐arid regions is becoming more important. Exchangeable K+, determined by ammonium acetate (NH4OAc), might not be the best predictor of the soil K+ available to crops in soils containing micaceous minerals. The effectiveness of different extraction methods for the prediction of K‐supplying capacities and quantity–intensity relationships was studied in 10 calcareous soils in western Iran. Total K+ uptake by wheat grown in the greenhouse was used to measure plant‐available soil K+. The following methods extracted increasingly higher average amounts of soil K+: 0.025 M H2SO4 (45 mg K+ kg?1), 1 M NaCl (92 mg K+ kg?1), 0.01 M CaCl2 (104 mg K+ kg?1), 0.1 M BaCl2 (126 mg K+ kg?1), and 1 M NH4OAc (312 mg K+ kg?1). Potassium extracted by 0.01 M CaCl2, 1 M NaCl, 0.1 M BaCl2, and 0.025 M H2SO4 showed higher correlation with K+ uptake by the crop (P < 0.01) than did NH4OAc (P < 0.05), which is used to extract K+ in the soils of the studied area. There were significant correlations among exchangeable K+ adsorbed on the planar surfaces of soils (labile K+) and K+ plant uptake and K+ extracted by all extractants. It would appear that both 0.01 M CaCl2 and 1 M NaCl extractants and labile K+ may provide the most useful prediction of K+ uptake by plants in these calcareous soils containing micaceous minerals.  相似文献   

3.
Abstract

The potassium (K) supplying capacity of a deeply weathered profile developed over granite from Peninsular Malaysia was investigated by employing the quantity‐intensity (Q/I) approach. The values of potential buffering capacity (PBCK), labile K (KL), specific K (KO), and specific K sites (KX) were considerably higher in the saprolite zones as compared to the solum layers. This indicated that depletion of K on cropping would be faster in the solum materials than in the saprolites. Potassium equilibrium activity ratio was in the sequence: solum > middle saprolite > upper saprolite. Free energy values showed low, but sufficient, level of available K reserve in this profile. The relationships of Q/I parameters with physico‐chemical characteristics and clay mineralogy of the profile were discussed. The changes in the Q/I parameters as a function of depth were found to be associated with the contents of clay and organic matter in the solum, while in the saprolites, the clay mineralogy which composed mainly of K‐feldspar, mica, and mica‐smectite seemed to be the main factor.  相似文献   

4.
Abstract

In order to calculate the potassium (K) fertilizer requirement, it is necessary to know how much of this nutrient element must be applied in order to overcome any buffering effects and raise the soil test value to a desired level. A glasshouse study was conducted on a wide range of KwaZulu‐Natal (South Africa) soils to establish this information. The topsoil (0–200 mm) at 51 sites was sampled. Soils varied greatly in texture (4–83% clay), organic carbon (0.2–9.2%), and clay mineralogy (kaolinitic‐sesquioxic through to illitic and smectitic). Soil from each site was treated with four levels of K and taken through three wetting and drying cycles over a six‐week period. Analysis for K using the “Ambic”; [ammonium bicarbonate (NH4HCO3)/ammonium fluoride (NH4F)/EDTA] extractant showed that the quantity of applied K (kg ha‐1) required to raise the soil test value by a unit (1 mg L‐1), i.e., the K requirement factor, varied between 1.5 and 8.8. Therefore, on soils that display the highest K fixation, the calculated fertilizer K requirement, which is currently based on a factor of 2.5, could be underestimated by as much as 70%. Clay mineral analysis showed that the higher levels of K fixation tended to be associated with the presence of vermiculite.  相似文献   

5.
This investigation was done to determine the release of potassium (K) from five calcareous soils of southern Iran using 0.025 M CaCl2, HCl and citric acid during six successive extractions and to study the K fixation capacity of the soils after K release experiment. Mineralogical study indicated that Vertisols and Mollisols were dominated with smectites; while other soils had illite, chlorite, palygorskite and smectite. Results indicated that citric acid extracted more K than CaCl2 and HCl (137 vs. 111 and 113 mg kg?1, respectively). The analysis of calcium (Ca), magnesium (Mg) and K concentrations in the solutions suggests that the exchange of K with soluble Ca and Mg (originated from dissolution of carbonates by acidic solutions) is the main mechanism of K release, but citrate is able to dissolve K-bearing minerals and release K in slightly calcareous soils. Soils with more illite released more K. Potassium fixation capacity of soils increased after extractions of soils with different extractants from 324 to 471 mg kg?1, with no significant difference. It is suggested to apply more K fertilizers in K-depleted calcareous soils and use of different solutions for extracting K from soil minerals may be a temporary and short term solution.  相似文献   

6.
ABSTRACT

We studied (i) the pH buffer capacity (pHBC) of calcareous soils varied widely in calcite and texture, (ii) the contribution of soil properties to pHBC and (iii) the significance of using a model based on calcite dissolution to estimate the pHBC of calcareous soils. The pHBC of soils was measured by adding several rates of HCl to soils (100–6500 mM H+ kg–1), in a 0.01 M CaCl2 background and an equilibration time of 24 h. The pHBC (mM H+ kg–1 pH?1) varied from 55 to 3383, with the mean of 1073. The pHBC of the soils was strongly correlated with soil CaCO3 equivalent (calcite) (r = 0.94), sand (r = ?0.72), silt (r = 0.60), EC (r = 0.63), pH (r = 0.55), and weakly (r = 0.37) but significantly with clay content. The attained pHBC values indicated that calcite was probably the main buffer system in these soils. The chemical equilibrium model successfully predicted pH titration curves based on calcite dissolution, indicating buffering of acid inputs in the calcareous soils is dominated by calcite dissolution. The model can be used to simulate acidification of calcareous soils and to provide information for making environmental management decisions.  相似文献   

7.

Purpose

A laboratory incubation under constant temperature and humidity was conducted to estimate the impacts of nitrogen (N) fertilizers on the acidification of two acid soils (Plinthudult and Paleudalfs) in south China.

Materials and methods

The experiment had three treatments, i.e., control (CK), addition of urea (U), and addition of ammonium sulfate (AS). We measured soil pH, nitrate (NO3 ?), ammonium (NH4 +), exchangeable hydrogen ion (H+), and aluminum ion (Al3+) concentrations at various intervals during the 90 days of incubation. Soil buffering capacity (pHBC) was also measured at the end of the experiment.

Results and discussion

The application of N fertilizers resulted in soil acidification. The U treatment caused greater acidification of the Plinthudult soil than the AS treatment, while there were no differences between U and AS treatments on the acidification of the Paleudalfs. At the end of the trial, the pHBC of Plinthudult in AS treatment was greater than that in CK and U treatments, which may be due to the buffering system of NH4 + and NH4OH. However, the pHBC of Paleudalfs was unchanged between treatments. The dynamics of exchangeable H+ and Al3+ corresponded to that of soil pH. Correlation analysis showed that both soil exchangeable H+ and soil exchangeable Al3+ were significantly related to soil pH.

Conclusions

Application of urea and ammonium sulfate caused acidification in both soils and increased soil exchangeable Al3+ and H+ concentrations in the Paleudalfs. The application of urea increased exchangeable Al3+, and ammonium sulfate increased pHBC in the Plinthudult.  相似文献   

8.
Potassium (K+) directly released from primary K‐bearing minerals can contribute to plant nutrition. The objective of this research was to assess short‐term K+ release and fixation on a range of intensively cropped calcareous soils. Potassium sorption and desorption properties and the contributions of exchangeable‐K+ (EK) and nonexchangeable‐K+ (NEK) pools to K+ dynamics of the soil‐solution system was measured using a modified quantity‐to‐intensity (Q : I) experiment. Release and fixation of K+ were varied among soils. The relation between the change in the amount of NEK during the experiment and the initial constrain was linear, and soil ability for K+ release and fixation (β) for all soils varied from 0.041 to 0.183, indicating that 4% to 18% of added K+ converted to NEK when fixation occurred. The equilibrium potential buffering capacity (PBC) for K+ derived from Q : I experiments had significant correlation (r = 0.75, p < 0.01) with β, indicating that PBC depends not only on exchange properties but also on release and fixation properties. The depleted soils showed higher β value than the other soils, indicating much of the added K+ was converted to NEK in case of positive constraint. The range of the amount of EK which was not in exchange equilibrium with Ca (Emin) in the experimental conditions was large and varied from 0.68 to 9.00 mmol kg–1. On average, Emin amounted to 64% of EK. This fraction of EK may not be available to the plant. The parameters obtained from these short‐term K+ release and fixation experiments can be used in plant nutrition.  相似文献   

9.
Experiments were carried out to evaluate the dynamics of potassium (K) in six representative soil series of southwestern Nigeria to provide guidelines on soil K management. Quantity–intensity (Q/I) approach was used and the Q/I isotherms obtained revealed that all the soils released K before reaching equilibrium, having a negative intercept. The results showed that labile K from the Q/I evaluation was greater than exchangeable K from ammonium–acetate extraction in all the soils, showing that evaluation of soil K by exchangeable K alone may not give an in-depth understanding of the K dynamics in soil. Hence, it should be used in addition to Q/I parameters for a reliable evaluation. The potential buffering capacity obtained ranged from 0.4983 to 1.4272 cmol kg?1/(mol L?1)1/2, indicating that the soils have a low capacity to maintain K concentration for a long period and hence would require frequent K fertilization.  相似文献   

10.
ABSTRACT

Quantity-Intensity (Q/I) parameters were used for elucidating the role of buffering properties of soils through K depletion. Winter wheat was sown in a greenhouse pot experiment until K-depletion and soils were analyzed with NH4OAc and NaBPh4 (1 min incubation period). Q/I isotherms (partitioned in exchangeable and non-exchangeable form) were constructed for the soils before and at the end of the K-exhaustion experiment. Results showed that NaBPh4-K correlated better than NH4OAc-K with intensity parameter (AReK) or labile K (-ΔΚ0) in K-depleted soils (r = 0.41 and 0.70), indicating the importance of non-exchangeable K in K dynamics. The latter was confirmed from the comparison of buffering characteristics between initial and K-depleted soils which showed that among the soils studied there was a group whose increase in buffering capacity (PBCKt) was due to non-exchangeable K fixation. Furthermore, NaBPh4-K was well predicted by the sum of exchangeable K and the quantity of K that has to be applied to achieve K balance as derived from Q/I isotherms (EK0 + CK0). Finally, relationships were found between Q/I parameters of the initial soils (-ΔΚ0i, ΕΚ0i, ΕΚri, CK0i) and the K-depleted ones (ΕΚrd, ΕΚ0d, CK0d, CKrd) which allowed corresponding prediction of the initial parameters (r2 = 0.78–0.87).  相似文献   

11.
Fate of fertilizer ammonium in soils with different composition of clay minerals in an incubation experiment In an incubation experiment with three different soils (gray brown podsolic soil from loess, alluvial gley, and brown earth, derived from basalt) the specific adsorption (fixation) and release of fertilizer NH4+ was investigated. In one treatment 120 mg NH4–N/kg soil was added, while the other treatment (control) received no nitrogen. Soils samples were taken every ten days and analyzed for nonexchangeable and exchangeable NH4+ and NO3?. The experimental results are showing that the specific adsorption of applied NH4+ was related to the type of clay minerals. While the loess soil, rich in illite, and the alluvial soil, rich in expansible clay minerals, bound about 40% of the added NH4+ specifically, the soil derived from basalt with mainly kaolinite bound only about 10 %. From the recently “fixed” fertilizer NH4+ about a half was nitrified during the incubation period of about 9 weeks. In the control there was no significant release of specifically bound NH4+. Obviously this NH4+ is located more deeply in the interlayers of the clay minerals and not available to microorganisms.  相似文献   

12.
A study was conducted at two experimental tree plantations in the Pacific Northwest to assess the roles of bacteria and fungi in nitrogen (N) cycling. Soils from red alder (Alnus rubra) and Douglas-fir (Pseudotsuga menziesii) plots in low- (H.J. Andrews) and high- (Cascade Head) productivity stands were sampled in 2005 and 2006. Fungal:bacterial ratios were determined using phospholipid fatty acid (PLFA) profiles and quantitative (Q)-PCR. Ratios from these two molecular methods were highly correlated and showed that microbial biomass varied significantly between the two experimental sites and to a lesser extent between tree types with fungal:bacterial biomass ratios lower in more N-rich plots. 15N isotope dilution experiments, with ammonium (NH4+) and nitrate (NO3?), were paired with antibiotics that blocked bacterial (bronopol) and fungal (cycloheximide) protein synthesis. This modified isotope dilution technique was used to determine the relative contribution of bacteria and fungi to net N mineralization and gross rates of ammonification and nitrification. When bacterial protein synthesis was blocked NH4+ consumption and nitrification rates decreased in all treatments except for NH4+ consumption in the Douglas-fir plots at H.J. Andrews, suggesting that prokaryotic nitrifiers are a major sink for mineral NH4+ in forest soils with higher N availability. Cycloheximide consistently increased NH4+ consumption, however the trend was not statistically significant. Both antibiotics additions also significantly increased gross ammonification, which may have been due to continued activity of extra- and intracellular enzymes involved in producing NH4+ combined with the inhibition of NH4+ assimilation into proteins. The implication of this result is that microorganisms are likely a major sink for soil dissolved organic N (DON) in soils.  相似文献   

13.
太湖地区主要土壤中的固定态铵及其有效性   总被引：7，自引：1，他引：7  
测定了太湖地区主要土壤中固定态铵的储量和表土的固铵能力,并通过盆栽试验研究了它们的有效性。土壤的固定态铵含量和表土的固铵能力因母质而异,长江冲积物发育的土壤最高,次为黄土状物质的,第四纪红色粘土的最低。各土壤0—20厘米土层中的固定态铵总量平均占全氮总量的18.5%,0—100厘米土体中占34%。各土壤“固有的”固定态铵的有效性差异较大,视土层等的不同,在0—13%间。“新固定”的来自肥料或土壤有机质矿化释出的铵则很高,一般均能被当季作物完全吸收利用。渍水条件并不能提高固定态铵的有效性。讨论了铵的固定作用在土壤氮素肥力中的意义;指出,由于铵的固定作用和不同土壤的固铵能力各异,常用的淹水培育法所得到的土壤氮素矿化量值不但一般偏低,而且难于进行相互比较。  相似文献   

14.
Reliable and quick methods for measuring nitrogen (N)–supplying capacities of soils (NSC) are a prerequisite for using N fertilizers. This study was conducted to develop a routine method for estimation of mineralizable N in two calcareous soils (sandy loam and clay soils) treated with municipal waste compost or sheep manure. The methods used were anaerobic biological N mineralization, mineral N released by 2 M potassium chloride (KCl), ammonium (NH4 +) N extracted by 1 N sulfuric acid (H2SO4), NH4 +-N extracted by acid potassium permanganate (KMnO4), and NH4 +-N released by oxidation of soil organic matter using acidified potassium permanganate. The results showed that oxidizable N extracted by acid permanganate, a simple and rapid measure of soil N availability, was correlated with results of the anaerobic method. Oxidative 0.05 N KMnO4 was the best method, accounting for 78.4% of variation in NSC. Also, the amount of mineralized N increased with increasing level of organic materials and was greater in clay soil than sandy loam soil.  相似文献   

15.
盆栽和田间条件下土壤15N标记肥料氮的转化   总被引：14，自引：2，他引：14  
程励励  文启孝  李洪 《土壤学报》1989,26(2):124-130
利用15N在盆栽条件下研究了铵的矿物固定作用对肥料氮在三种土壤中转化的影响.结果表明,红壤性水稻土不固定肥料铵,但在白土和夹沙土中,56-77%的肥料氮被土壤矿物所固定,这些“新固定”的固定态铵的有效性很高,其中90%以上在30-50天内即被水稻所吸收,或者为微生物所利用转变为生物固定态氮.生物固定态氮对当季作物的有效性远较“新固定”的固定态铵的低.田间微区试验的结果还表明,甚至第二、三季作物吸收的残留肥料氮中,20-86%的氮也系来自固定态铵.作者认为,对具有较强固铵能力的土壤来说,只有了解铵的矿物固定作用,才能正确了解肥料氮的其它转化过程.  相似文献   

16.
Data on the mineralogical composition of clay in soils of solonetzic complexes of the Priobskoe Plateau and the Kulunda and Baraba lowlands have been generalized. The parent materials predominating in these regions have loamy and clayey textures and are characterized by the association of clay minerals represented by dioctahedral and trioctahedral mica–hydromica, chlorite, kaolinite, and a number of irregular interstratifications. They differ in the proportions between the major mineral phases and in the qualitative composition of the minerals. Mica–hydromica and chlorites with a small amount of smectitic phase predominate on the Priobskoe Plateau and in the Kulunda Lowland; in the Baraba Lowland, the portion of mica–smectite interstratifications is higher. An eluvial–illuvial distribution of clay fraction in solonetzes is accompanied by the acid–alkaline destruction and lessivage of clay minerals, including the smectitic phase in the superdispersed state. This results in the strong transformation of the mineralogical composition of the upper (suprasolonetzic) horizons and in the enrichment of the solonetzic horizons with the products of mineral destruction; superdispersed smectite; and undestroyed particles of hydromica, kaolinite, and chlorite from the suprasolonetzic horizons. A significant decrease in the content of smectitic phase in the surface solodic horizons of solonetzic complexes has different consequences in the studied regions. In the soils of the Priobskoe Plateau and Kulunda Lowland with a relatively low content (10–30%) of smectitic phase represented by chlorite–smectite interstratifications, this phase virtually disappears from the soils (there are only rare cases of its preservation). In the soils of the Baraba Lowland developed from the parent materials with the high content (30–50%) of smectitic phase represented by mica–smectite interstratifications, the similar decrease (by 10–20%) in the content of smectitic phase does not result in its complete disappearance. However, the smectitic phase acquires the superdispersed state and the capacity for migration.  相似文献   

17.
湖南几种耕地土壤固定添加铵的动力学研究   总被引：2，自引：0，他引：2  
通过野外调查取样、室内培养试验和分析测定，研究了湖南省几种成土母质发育的旱地土壤和稻田土壤固定添加铵的动力学特性。结果表明，供试土壤对添加铵的固定速度很快，尤其在反应的前8～12h内速度更快，12h后速度逐渐变慢，24h以后，土壤对外源铵的固定已基本达到平衡。数学拟合表明，一级动力学方程和Elovich方程两种动力学模型能较好地拟合供试土壤固定添加铵的动力学特性，经统计均达极显著水平，抛物扩散方程也有较好的拟合效果，零级方程较差。由一级动力学方程求得的不同土壤固铵动力学参数：理论最大固铵量（A）、反应速率常数（b）以及反应半时值明显不同。耕型石灰性紫色土、耕型酸性紫色土、耕型棕色石灰土和耕型石灰岩红壤的理论最大固铵量和反应半时值分别为212．3mg kg^-1、179．0mg kg^-1、142．9mg kg^-1.13．7mg kg^-1和29．75h、25．96h、27．18h、23．49h；紫泥田、河沙泥、灰泥田和红黄泥的理论最大固铵量和反应半时值分别为86．2mg kg^-1、68．7mg kg^-1,31．8mg kg^-1、19．1mg kg^-1和14．50h、15．10h、15．51h、18．43h。耕型石灰性紫色土、耕型酸性紫色土、耕型棕色石灰土和耕型石灰岩红壤的反应速率常数分别为0．0233 h^-1、0．0267h^-1、0．0255h^-1、0．0295h^-1；紫泥田、河沙泥、灰泥田和红黄泥的反应速率常数分别为0．0478h^-1、0．0459h^-1、0．0447h^-1、0．0376h^-1.除耕型石灰岩红壤以外，旱地土壤的理论最大固铵量和反应半时值均明显大于水田土壤，而反应速率常数明显小于水田土壤。  相似文献   

18.
The correlation of soil temperature and moisture with inorganic N concentrations and net mineralization beneath major species types in mature boreal and northern hardwood forests was examined over a two year period. Soils beneath species types where the canopy was dominated byBetula papyrifera, Picea glauca, Alnus rugosa or, in northern hardwoods,Acer saccharum were studied. Net NO3 ? mineralization varied by species type and net total inorganic nitrogen (N) mineralization varied by month and the interaction of species type with month. Soil NO3 ? concentration and NO3 ? mineralization were correlated for spruce, and inversely correlated for alder and maple. Soil NH4 + concentration and NH4 + mineralization were inversely correlated for alder and maple. In laboratory temperature and moisture treatments of birch, spruce and maple soils, NH4 + and total inorganic N-mineralization increased with temperature. The response to moisture was most evident for NO3 ? mineralization in maple soils.  相似文献   

19.
A soil column method was used to compare the effect of drip fertigation (the application of fertilizer through drip irrigation systems, DFI) on the leaching loss and transformation of urea-N in soil with that of surface fertilization combined with flood irrigation (SFI), and to study the leaching loss and transformation of three kinds of nitrogen fertilizers (nitrate fertilizer, ammonium fertilizer, and urea fertilizer) in two contrasting soils after the fertigation. In comparison to SFI, DFI decreased leaching loss of urea-N from the soil and increased the mineral N (NH4+-N + NO3--N) in the soil. The N leached from a clay loam soil ranged from 5.7% to 9.6% of the total N added as fertilizer, whereas for a sandy loam soil they ranged between 16.2% and 30.4%. Leaching losses of mineral N were higher when nitrate fertilizer was used compared to urea or ammonium fertilizer. Compared to the control (without urea addition), on the first day when soils were fertigated with urea, there were increases in NH4+-N in the soils. This confirmed the rapid hydrolysis of urea in soil during fertigation. NH4+-N in soils reached a peak about 5 days after fertigation, and due to nitrification it began to decrease at day 10. After applying NH4+-N fertilizer and urea and during the incubation period, the mineral nitrogen in the soil decreased. This may be related to the occurrence of NH4+-N fixation or volatilization in the soil during the fertigation process.  相似文献   

20.
The aim of this study was to investigate the influence of four different horticultural management practices in open field and in greenhouse conditions under organic and conventional cultivation on the amount of soluble organic nitrogen (SON) present in the soil. Soils used in greenhouses and open field cultivation were sampled in Shanghai, China, where organic farming has been conducted for 3 years or conventional faming has been continued in the same area. The amounts of SON, nitrate (NO3?) and ammonium (NH4+) were greater in the greenhouse soils than those under open field cultivation, which indicated a higher degree of soil management was imposed under greenhouse conditions. Greenhouse cultivation is also known to accelerate the turnover of SON in the soils, which may explain the significantly higher amounts of SON present in these soils. Organic farming, which does not use artificial fertilizers and pesticides, also resulted in significantly higher amounts of SON (average 42.10 mg kg?1) compared with soils under conventional faming (24.59 mg kg?1). The reasons for the observed differences in pool sizes of soluble inorganic nitrogen (SIN) and NO3? in the greenhouse soils and the open fields include (a) the heavy application of both complex fertilizer and organic fertilizer that exceeded crop requirements and (b) warmer temperatures and moist soils in the greenhouses, which are likely to lead to greater rates of N cycling compared with the open field soils. These results suggest that SON may be an important source of N in all horticultural systems, representing a pool of labile N readily available for plant growth. However, its concentration is less sensitive to different management practices than SIN. In contrast to SON, the total soluble nitrogen and inorganic N (SIN) pools varied widely with the different management practices although they were dominated by NO3? in all treatments. Soil organic N was positively related to dissolved organic carbon and NO3? contents. This relationship indicates that NO3? and dissolved organic matter play a key role in the retention of SON in soil.  相似文献   

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