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1.

Purpose

Understanding hydro-sedimentary dynamics at the catchment scale requires high temporal resolution data on suspended sediments such as their origin, in addition to the common measurements of sediment concentrations and discharges. Some rapid and low-cost fingerprinting methods based on spectroscopy have recently been developed. We investigated how visible spectra could be used to predict the proportion of various source materials in suspended sediment samples, paying particular attention to the potential alteration of spectrocolorimetric signatures between soils and suspended sediments during transport.

Materials and methods

The 22-km2 Galabre catchment, France, is composed of black marls, limestones, molasses, undifferentiated deposits and gypsum. Forty-eight source materials were sampled and 328 suspended sediment samples were collected at the outlet during 23 runoff events. Measurements were taken with a diffuse reflectance spectrophotometer on dried samples. As the erosion processes are particle size selective, five particle size fractions of source material were measured in order to assess the potential alteration of the fingerprint signatures. As the biogeochemical processes occurring in the river could also affect the signatures, source materials were immersed in the river for durations ranging from 1 to 63 days and subsequently measured. Finally, partial least-squares regression models were constructed on 81 artificial laboratory mixtures to predict the proportions of source materials.

Results and discussion

The spectrocolorimetric measurements discriminated the primary source materials but not the Quaternary deposits. As the gypsum was not conservative, only the black marls, molasses and limestones were used in the fingerprinting procedure. The construction of the partial least-squares regression models led to a median absolute error of 1.1%. This error increased to 3.9% when the models were applied to source samples with: (1) different particle sizes; (2) different durations spent in the river; or (3) different origins than those used for their construction. The effect of particle size on the fingerprinting procedure was larger than the effect of biogeochemical reactions or the spatial variability of the spectrocolorimetric signatures. Half of the 23 runoff events analysed exhibited huge variations in the source proportions from one sediment sample to another.

Conclusions

The spectrocolorimetric fingerprinting approach was able to quantify routinely the proportion of primary source materials in all suspended sediment samples collected during runoff events. The high temporal resolution of the predicted proportions revealed that only analysing three or four suspended sediment samples during a runoff event could lead to a misunderstanding of the hydro-sedimentary processes for more than half of the investigated runoff events.  相似文献   

2.

Purpose

Knowledge of sediment sources is a prerequisite for sustainable management practices and may furthermore improve our understanding of water and sediment fluxes. Investigations have shown that a number of characteristic soil properties can be used as “fingerprints” to trace back the sources of river sediments. Spectral properties have recently been successfully used as such characteristics in fingerprinting studies. Despite being less labour-intensive than geochemical analyses, for example, spectroscopy allows measurements of small amounts of sediment material (>60 mg), thus enabling inexpensive analyses even of intra-event variability. The focus of this study is on the examination of spectral properties of fluvial sediment samples to detect changes in source contributions, both between and within individual flood events.

Materials and methods

Sediment samples from the following three different origins were collected in the Isábena catchment (445 km2) in the central Spanish Pyrenees: (1) soil samples from the main potential source areas, (2) stored fine sediment from the channel bed once each season in 2011 and (3) suspended sediment samples during four flood events in autumn 2011 and spring 2012 at the catchment outlet as well as at several subcatchment outlets. All samples were dried and measured for spectral properties in the laboratory using an ASD spectroradiometer. Colour parameters and physically based features (e.g. organic carbon, iron oxide and clay content) were calculated from the spectra. Principal component analyses (PCA) were applied to all three types of samples to determine natural clustering of samples, and a mixing model was applied to determine source contributions.

Results and discussion

We found that fine sediment stored in the river bed seems to be mainly influenced by grain size and seasonal variability, while sampling location—and thus the effect of individual tributaries or subcatchments—seem to be of minor importance. Suspended sediment sources were found to vary between, as well as within, flood events; although badlands were always the major source. Forests and grasslands contributed little (<10 %), and other sources (not further determinable) contributed up to 40 %. The analyses further suggested that sediment sources differ among the subcatchments and that subcatchments comprising relatively large proportions of badlands contributed most to the four flood events analyzed.

Conclusions

Spectral fingerprints provide a rapid and cost-efficient alternative to conventional fingerprint properties. However, a combination of spectral and conventional fingerprint properties could potentially permit discrimination of a larger number of source types.  相似文献   

3.

Purpose

Knowledge of the origin of suspended sediment is important for improving our understanding of sediment dynamics and thereupon support of sustainable watershed management. An direct approach to trace the origin of sediments is the fingerprinting technique. It is based on the assumption that potential sediment sources can be discriminated and that the contribution of these sources to the sediment can be determined on the basis of distinctive characteristics (fingerprints). Recent studies indicate that visible–near-infrared (VNIR) and shortwave-infrared (SWIR) reflectance characteristics of soil may be a rapid, inexpensive alternative to traditional fingerprint properties (e.g. geochemistry or mineral magnetism).

Materials and methods

To further explore the applicability of VNIR-SWIR spectral data for sediment tracing purposes, source samples were collected in the Isábena watershed, a 445 km2 dryland catchment in the central Spanish Pyrenees. Grab samples of the upper soil layer were collected from the main potential sediment source types along with in situ reflectance spectra. Samples were dried and sieved, and artificial mixtures of known proportions were produced for algorithm validation. Then, spectral readings of potential source and artificial mixture samples were taken in the laboratory. Colour coefficients and physically based parameters were calculated from in situ and laboratory-measured spectra. All parameters passing a number of prerequisite tests were subsequently applied in discriminant function analysis for source discrimination and mixing model analyses for source contribution assessment.

Results and discussion

The three source types (i.e. badlands, forest/grassland and an aggregation of other sources, including agricultural land, shrubland, unpaved roads and open slopes) could be reliably identified based on spectral parameters. Laboratory-measured spectral fingerprints permitted the quantification of source contribution to artificial mixtures, and introduction of source heterogeneity into the mixing model decreased accuracies for some source types. Aggregation of source types that could not be discriminated did not improve mixing model results. Despite providing similar discrimination accuracies as laboratory source parameters, in situ derived source information was found to be insufficient for contribution modelling.

Conclusions

The laboratory mixture experiment provides valuable insights into the capabilities and limitations of spectral fingerprint properties. From this study, we conclude that combinations of spectral properties can be used for mixing model analyses of a restricted number of source groups, whereas more straightforward in situ measured source parameters do not seem suitable. However, modelling results based on laboratory parameters also need to be interpreted with care and should not rely on the estimates of mean values only but should consider uncertainty intervals as well.  相似文献   

4.

Purpose

The importance of bank erosion was quantified during three periods (October 2006–April 2007, May 2007–April 2008 and May 2008–April 2009) in the 486 km2 catchment area of River Odense, Denmark. A catchment sediment budget was established including other sediment sources such as tile drains and surface runoff, in-channel and overbank sinks and storage and the resulting bed load and suspended sediment load exported from the catchment.

Material and methods

Bank erosion and sedimentation were measured using ca. 3,000 erosion pins established in 180 pin plots, each consisting of three vertical lines of pins. Thirty-six representative reaches, each with a length of 100 m, were selected by a stratified random procedure in GIS. Bed load and suspended sediment export from the catchment were measured using a bed load sampler and from continuous measurements of turbidity at the outlet gauging station.

Results and discussion

The gross sediment input from bank erosion during the three study periods amounted to 21,100–25,200 t in the River Odense catchment, which is considerably higher than the estimated input of sediment from tile drains and surface runoff, which amounted to 220–500 t and 0–100 t, respectively. The measured bed load (20–490 t) was five to 60 times lower than the suspended sediment export from the catchment (1,240–2,620 t) during the three study periods, with the largest difference occurring in the driest year. Sediment sinks and storage were of high importance for the catchment sediment budget as the measured in-channel storage of sediment on stream banks was as high as 16,200–20,100 t, and the overbank sediment sink was estimated at 360–3,100 t.

Conclusions

Bank erosion was the dominant sediment source (90–94 %) in the River Odense catchment during the three study years. In-channel and overbank sediment sinks and storage dominated the sediment budget as 79–94 % of the sediment input from all sources was not exported from the catchment during the three study years. Such a large attenuation of sediment in river channels and on floodplains is extremely important for fluvial habitats and ecology. Moreover, it has strong implications for attempts to document changes in sediment export following implementation of mitigation measures.  相似文献   

5.

Purpose

We employ a geochemical-fingerprinting approach to estimate the source of suspended sediments collected from tributaries entering Falls Lake, a 50-km2 drinking water reservoir on the Neuse River, North Carolina, USA. Many of the major tributaries to the lake are on North Carolina’s 303(d) list for impaired streams, and in 2008, the lake was added to that list because of high values of turbidity, likely sourced from tributary streams.

Materials and methods

Suspended sediments were collected from four streams with a time-integrated sampler during high-flow events. In addition, composite sediment samples representing potential sources were collected from stream banks, forests, pastures, construction sites, dirt and paved roads, and road cuts within tributary basins. Radiocarbon dating and magnetic susceptibility measurements were used to determine the origin of stream bank alluvial deposits. Sediment samples were analyzed for the concentrations of 55 elements and two radionuclides in order to identify tracers capable of distinguishing between potential sediment sources. The relative sediment source contributions were determined by applying a Monte Carlo simulation that parameterized the geochemical tracer data in a mixing model.

Results and discussion

Radiocarbon and magnetic susceptibility measurements confirmed the presence of “legacy” sediment in the Ellerbe and New Light Creek valley bottoms. Mixing model results demonstrate that stream bank erosion is the largest contributor to the suspended sediment load in New Light Creek (62%), Ellerbe Creek (58%), and Little Lick Creek (33%), and is the second largest contributor in Lick Creek (27%) behind construction sites (43%).

Conclusions

We find that stream bank erosion is the largest nonpoint source contributor to the suspended sediment load in three of the four catchments and is therefore a significant source of turbidity in Falls Lake. The presence of legacy sediment appears to coincide with increased contributions from stream bank erosion in Ellerbe and New Light creeks. Active construction sites and timber harvesting were also significant sources of suspended sediment. Water quality mitigation efforts need to consider nonpoint-source contributions from stream bank erosion of valley bottom sediments aggraded after European settlement.  相似文献   

6.

Purpose

There is a growing interest in the characterization of the particle size of sediment due to its impact on particle dynamics, especially for connectivity purpose. This study determined the particle size distribution of suspended sediment in a mountainous catchment, with the aim to evaluate the variability of particle size during floods, the main controlling factors, and if indirect information from hillslopes was useful for the interpretation of particle size measured at the catchment outlet. This work involved the development of a measurement protocol.

Material and methods

Samples were collected automatically from streamwater during flood events using an ISCO 3700 sampler. Five events were analyzed for their particle size distributions using a Malvern Mastersizer 2000. Because the samples were too concentrated, two different protocols were tested to address the errors made during the subsampling step: using a pipette and a home-made device with successive dilution phases.

Results and discussion

High errors occurred when using a pipette to extract particles within a stirred sample. The maximum errors were reduced from 1,600 to 30?% using the device described within this study. Particles were found to be aggregated at various levels regardless of the discharge they were sampled at. Their size was found to be either variable or stable at the event scale, and statistical analyses revealed that discharge was the factor that best correlated with particle size. The results obtained in this study are in agreement with the few other studies in comparable environments. Some hypothesis are put forward and discussed to explain the positive relationship between particle size and discharge. Input from hillslopes seems to have a measureable effect in this headwater catchment.

Conclusions

While the need for in situ measurements has long been stressed in lowland rivers, estuaries, and coastal environments, it was shown that the use of an accurate dilution protocol could provide some physically interpretable measurements on the particle size distributions of suspended sediment transported in a mountainous catchment. It also appears that hillslope information has to be considered when studying particle size measured at the catchment outlet.  相似文献   

7.

Purpose

Quantifying suspended sediment fluxes and dynamics across mountains, and identifying the origin of sediment in severely eroded areas, are of primary importance for the management of water resources. This contribution aims to generalise previous results from suspended sediment fingerprinting obtained during 2007?C2009 in a mesoscale Alpine catchment (the Bléone River; 905?km2) in France, and to assess variability in sediment sources throughout the second half of the twentieth century.

Materials and methods

Sediment fingerprinting, based on elemental geochemistry and radionuclide measurements, was conducted on a sediment core collected in an alluvial floodplain at the basin outlet. This technique was combined with hydro-sedimentary time-series to reconstruct the origin of suspended sediment deposited at this location over the last 50?years.

Results and discussion

Interpretation of sedimentation based on historical hydrological databases corroborates core dating obtained with 137Cs and 210Pbxs activity measurements. Black marls and (marly) limestone sources provided the main fraction of sediment throughout the sequence (40 and 22?%, respectively). However, we also found evidence for the occurrence of major floods carrying large quantities of sediment originating from Quaternary deposits and conglomerates (25 and 16?%, respectively). The variability of sediment sources throughout the sequence may reflect the spatial variability of rainfall within the catchment, which in turn reflects its origin. However, the relatively homogeneous sediment composition throughout the sequence confirms that core-derived information is representative of widespread flood events.

Conclusions

These results are consistent with those obtained in previous studies. They also outline the need to take into account the entire grain size range of fine sediment in order to provide an overall picture of sediment sources and transfers within highly erosive catchments. This study also emphasizes the importance of using archival data to validate the results of sediment fingerprinting studies conducted during short contemporary monitoring programmes, and to extend fingerprinting of sediment sources over longer time-scales which include large and widespread floods.  相似文献   

8.

Purpose

Approximately 74 % of agricultural soils in Tunisia are affected by water erosion, leading to the siltation of numerous human-made reservoirs and therefore a loss of water storage capacity. The objective of this study was to propose a methodology for estimating the relative contributions of gully/channel bank erosion and surface topsoil erosion to the sediment accumulated in small reservoirs.

Materials and methods

We tested an approach based on the sediment fingerprinting technique for sediments collected from a reservoir (which has been in operation since 1994) at the outlet of a catchment (Kamech, 2.63 km2). Sampling concentrated on the soil surface (in both cropland and grassland), gullies and channel banks. A total of 17 sediment cores were collected along a longitudinal transect of the Kamech reservoir to investigate the origin of the sediment throughout the reservoir. Radionuclides (particularly caesium-137, 137Cs) and nutrients (total phosphorus, total nitrogen and total organic carbon (TOC)) were analysed as potential tracers.

Results and discussion

The applications of a mixing model with 137Cs alone or 137Cs and TOC provided very similar results: The dominant source of sediment was surface erosion, which was responsible for 80 % of the total erosion within the Kamech catchment. Additionally, we showed that the analysis of a single composite core provided information on the sediment origin that was consistent with the analysis of all sediment layers in the core. We demonstrated the importance of the core sampling location within the reservoir for obtaining reliable information regarding sediment sources and the dominant erosion processes.

Conclusions

The dominance of surface erosion processes indicates that conservation farming practices are required to mitigate erosion in the agricultural Kamech catchment. Based on the results from 17 sediment cores, guidelines regarding the number and location of sampling cores to be collected for sediment fingerprinting are proposed. We showed that the collection of two cores limited the sediment source apportionment uncertainty due to the core sampling scheme to <10 %.  相似文献   

9.

Purpose

Sediments adversely impact the quality of surface waters and are a significant source of contaminants, such as nutrients and pesticides, in agricultural watersheds. The development of effective beneficial management practices (BMPs) to minimize these impacts requires a sound understanding of the sources of sediments. The objectives of this study were: (1) to determine the sources of sediment in an agricultural watershed in the Canadian prairies using sediment source fingerprinting and; (2) to assess the results of the sediment fingerprinting study within the context of the scale of observation and the hydro-geomorphic connectivity of the watershed.

Materials and methods

Geochemical and radionuclide fingerprints were used to discriminate between the three potential sediment sources identified: topsoil, streambanks, and shale bedrock. Suspended and bed sediment samples were collected over the course of 3 years at six locations along the main stem of the creek, ranging from 3rd- (48 ha) to 7th-order (7441 ha) drainage basins. Four sediment fingerprint properties were selected that met statistical- and process-based selection criteria and the Stable Isotope Analysis in R model was used to estimate the proportion of sediment derived from each source at each sampling location in the watershed.

Results and discussion

The suspended sediments in the upper reaches were dominated by topsoil sources (64%–85%), whereas the suspended sediments moving through the lower reaches and being exported from the watershed had a higher proportion of sediment coming from streambank (32%–51%) and shale bedrock (29%–40%) sources. The switch in the sources of sediment between the headwaters and the watershed outlet are due to: (1) changes in sediment storage and connectivity; (2) a transition in the dominant erosion processes from topsoil to streambank erosion; and (3) the incision of the stream through the shale bedrock as it crosses the Manitoba Escarpment.

Conclusions

The results of this sediment fingerprinting study demonstrated that there was a switch in sediment sources between the headwaters and the outlet of the watershed. This research highlights the importance of the sampling location, in relation to the scale and geomorphic connectivity of the watershed, on the interpretation of results derived from the sediment fingerprinting technique, particularly in terms of developing suitable watershed BMPs to protect surface waters.  相似文献   

10.

Purpose

The study aimed to use the Soil and Water Assessment Tool (SWAT) model to simulate erosion processes in an alpine–prealpine catchment in order to provide data and information that may be relevant for managers so as to minimize reservoir siltation and water quality degradation. The main objective was to assess sediment production across the catchment and sediment supply to the main reservoir.

Materials and methods

The Barasona reservoir catchment (1,509 km2) is located in the Central Spanish Pyrenees, in the Ebro Basin. This catchment was selected for the case study given the regional significance of the Barasona reservoir and its siltation problems. The catchment has a mountain climate, with strong altitudinal and north–south gradients. The catchment is characterized by heterogeneous topography and lithology, resulting in a varied mosaic of slopes, soil types, and land covers. The Jueu karst system and two small headwater reservoirs were parameterized and calibrated in the model. The SWAT model sediment calibration for the catchment was based on a prior monthly hydrologic calibration, and the model validation was based on the sediment depositional history of the Barasona reservoir.

Results and discussion

The simulation period (2003–2006) and the validation period (1993–2002) produced average sediment yields to the reservoir of 643,000 and 575,000 t year?1, respectively. Large variations in sediment production were found between the subcatchments in the Barasona catchment due to differences in rock outcrops, land cover, and slope gradient. Sediment loss in the Jueu karst system was 15,500 t and the two small headwater reservoirs retained 31,200 and 50,300 t. Sediment production in relation to precipitation showed high temporal variability, with specific sediment yields to the Barasona reservoir ranging from 2.74 to 8.25 t ha?1 year?1. Strong lithological control was observed for sediment production in the subcatchments. The main sediment sources were located in the badlands developed on marls in the middle part of the catchment (internal depressions).

Conclusions

The proposed model has proved useful for identifying areas where significant erosion processes take place in large alpine–prealpine catchments at a regional level and also for assessing discharge losses by the karst system and the sedimentary role of the small reservoirs. The information obtained through this research will be of interest in assessing the spatial distribution of sediment sources and areas of high sediment yield, which will be useful to establish criteria for remediation strategies.  相似文献   

11.

Purpose

Sediment fingerprinting is a relatively recent research technique, capable of determining the origin of suspended sediment. In this study, we investigated sub-basins within a larger watershed we examined previously. The objectives were to determine if there was spatial variation in the origin of the suspended sediments and to test a streamlined fingerprinting approach which would reduce the cost, thereby paving the way for adoption by government agencies.

Materials and methods

Samples were collected from three tributaries, the outlet of the main stem, and at the middle of the main stem. Two methods to collect suspended sediment samples were compared: a mobile continuous-flow centrifuge and automated samplers. A relatively small initial tracer suite consisting of stable isotopes of nitrogen (N) and carbon (C) (15N and 13C), total N (TN), and total C (TC) was tested. Tracer concentrations were obtained through a single mass spectrometry analysis requiring <1 g of sediment.

Results and discussion

Multivariate discriminant analysis showed that three of the four tracers (δ 15N, δ 13C, and TC) from the initial pool were capable of accurate classification of the source samples. A multivariate mixing model showed that banks contributed the majority of sediment throughout all locations sampled and that in tributaries it was an even more dominant source. Despite variations in land use and stream order, the legacy sediments comprising the banks and floodplains were the main factor in impairment for suspended sediment. We found a small but statistically significant difference in δ 15N and δ 13C concentrations collected using automated samplers vs. the mobile centrifuge, but the effect on analysis of sediment source proportions was minimal.

Conclusions

The results of this study indicate that, at least in the study watershed, the majority of sediment in suspension was of streambank origin. A cost-effective tracer suite was identified as well as an attempt to make a streamlined approach to the technique. The streamlined approach cost much less ($7,550 US) than the conventional approach ($46,600 US) and should be suitable for total maximum daily loads analysis by state government agencies in the Southern Piedmont region of the USA.  相似文献   

12.

Purpose

Phosphorus (P) is a limiting nutrient for most US Midwestern aquatic systems and, therefore, increases of P, through point or non-point sources (NPS) of pollution such as agriculture, causes eutrophication. Identifying specific NPS contributions (e.g., upland vs. stream channels) for sediments and P is difficult due to the distributed nature of the pollution. Therefore, studies which link the spatial and temporal aspects of sediment and P transport in these systems can help better characterize the extent of NPS pollution.

Materials and methods

Our study used fingerprinting techniques to determine sources of sediments in an agricultural watershed (the North Fork of the Pheasant Branch watershed; 12.4 km2 area) in Wisconsin, USA, during the spring, summer, and fall seasons of 2009. The primary sources considered were uplands (cultivated fields), stream bank, and streambed. The model used fallout radionuclides, 137Cs, and 210Pbxs, along with total P to determine primary sediment sources. A shorter-lived fallout radioisotope, 7Be, was used to determine the sediment age and percent new sediments in streambed and suspended sediment samples (via the 7Be/210Pbxs ratio).

Results and discussion

Upland areas were the primary source of suspended sediments in the stream channels followed by stream banks. The sediment age and percent new sediment for the streambed and suspended sediments showed that the channel contained and transported newer (or more recently tagged with 7Be) sediments in the spring season (9–131 days sediment age), while relatively old sediments (165–318 days) were moving through the channel system during the fall season.

Conclusions

Upland areas are the major contributors to in-stream suspended sediments in this watershed. Sediment resuspension in stream channels could play an important role during the later part of the year. Best management practices should be targeted in the upland areas to reduce the export of sediments and sediment-bound P from agricultural watersheds.  相似文献   

13.
Analysis of sediment sources is an important component in the development of catchment sediment budgets and in determining links between erosion from sources and sediment delivery to catchment outlets. In this study 137Cs and 210Pbex were used to determine surface and sub-surface source contributions of fine sediment in a small upland headwater catchment (1.6 km2) in south-eastern Australia. The findings from this analysis are employed in an adjustment procedure to better differentiate sediment source erosion processes by utilising channel survey and erosion pin data. This improved the precision of estimates of sediment-source erosion-process contributions from hillslopes and channel/gully walls. A mean of 74% of in-channel deposits and suspended sediment exiting the study catchment was derived from sub-surface sources and when adjusted for erosion process this increased to 81%, which may be attributed to channel and gully wall erosion alone. Net erosion of the channel floor was low and constitutes only a small part of the total channel source input to sediment flux. Variability in sediment source contributions within the catchment was high, with rapid transition from hillslope to channel source dominance of sediment flux with distance downstream in the study catchment.  相似文献   

14.
Sediment budgets have been established for two small (<4 km2), lowland, agricultural catchments, by using 137Cs measurements, sediment source fingerprinting and more traditional monitoring techniques to quantify the individual components of the budget. The gross and net erosion rates for the fields on the catchment slopes were estimated using 137Cs measurements within selected fields, which encompassed a representative range of slope angles, slope lengths and land use. These estimates were extrapolated over the entire catchment, using a simple topographically driven soil erosion model (Terrain-Based GIS, TBGIS) superimposed on a DEM, to derive catchment average gross and net erosion rates. Suspended sediment yields were measured at the catchment outlets and sediment source fingerprinting techniques were used to establish the relative contributions from the catchment surface, subsurface tile drains and eroding channel banks to the sediment yields. In-channel and wetland storage were quantified using both direct measurements and 137Cs measurements. The sediment budgets established for the catchments highlighted the importance of subsurface tile drains as a pathway for sediment transfer, accounting for ca. 60% and 30% of the sediment output from the two catchments. Erosion from channel banks contributed ca. 10% and 6% of the sediment output from the two catchments. Although the suspended sediment yields from these catchments were considered high by UK standards (ca. 90 t km−2 year−1), the sediment delivery ratios ranged between 14% and 27%, indicating that a major proportion of the mobilised sediment was stored within the catchments. In-field and field-to-channel storage were shown to be of similar magnitude, but storage of sediment in the channel system and associated wetlands was relatively small, representing <5% of the annual suspended sediment yield.  相似文献   

15.

Purpose

The science of sediment fingerprinting has been evolving rapidly over the past decade and is well poised to improve our understanding, not only of sediment sources, but also the routing of sediment through watersheds. Here, we discuss channel–floodplain processes that may convolute or modify the sediment fingerprinting signature of alluvial bank/floodplain sources and explore the use of nonconservative tracers for differentiating sediment derived from surface soil erosion from that of near-channel fluvial erosion.

Materials and methods

We use a mathematical model to demonstrate the theoretical effects of channel–floodplain exchange on conservative and nonconservative tracers. Then, we present flow, sediment gauging data, and geochemical measurements of long- (meteoric beryllium-10, 10Be) and short-lived (excess lead-210 and cesium-137, 210Pbex and 137Cs, respectively) radionuclide tracers from two study locations: one above, and the other below, a rapidly incising knick zone within the Maple River watershed, southern Minnesota.

Results and discussion

We demonstrate that measurements of 10Be, 210Pbex, and 137Cs associated with suspended sediment can be used to distinguish between the three primary sediment sources (agricultural uplands, bluffs, and banks) and estimate channel–floodplain exchange. We observe how the sediment sources systematically vary by location and change over the course of a single storm hydrograph. While sediment dynamics for any given event are not necessarily indicative of longer-term trends, the results are consistent with our geomorphic understanding of the system and longer-term observations of sediment dynamics. We advocate for future sediment fingerprinting studies to develop a geomorphic rationale to explain the distribution of the fingerprinting properties for any given study area, with the intent of developing a more generalizable, process-based fingerprinting approach.

Conclusions

We show that measurements of conservative and nonconservative tracers (e.g., long- and short-lived radionuclides) can provide spatially integrated, yet temporally discrete, insights to constrain sediment sources and channel–floodplain exchange at the river network-scale. Fingerprinting that utilizes nonconservative tracers requires that the nonconservative behavior is predictable and verifiable.  相似文献   

16.

Purpose

Past metal mining has left a legacy of highly contaminated sediments representing a significant diffuse source of contamination to water bodies in the UK and worldwide. This paper presents the results of an integrated approach used to define the role of sediments in contributing to the dissolved lead (Pb) loading to surface water in a mining-impacted catchment.

Materials and methods

The Rookhope Burn catchment, northern England, UK is affected by historical mining and processing of lead ore. Quantitative geochemical loading determinations, measurements of interstitial water chemistry from the stream hyporheic zone and inundation tests of bank sediments were carried out.

Results and discussion

High concentrations of Pb in the sediments from the catchment, identified from the British Geological Survey Geochemical Baseline Survey of the Environment (GBASE) data, demonstrate both the impact of mineralisation and widespread historical mining. The results from stream water show that the stream Pb load increased in the lower part of the catchment, without any apparent or significant contribution of point sources of Pb to the stream. Relative to surface water, the interstitial water of the hyporheic zone contained high concentrations of dissolved Pb in the lower reaches of the Rookhope Burn catchment, downstream of a former mine washing plant. Concentrations of 56???g?l?1 of dissolved Pb in the interstitial water of the hyporheic zone may be a major cause of the deterioration of fish habitats in the stream and be regarded as a serious risk to the target of good ecological status as defined in the European Water Framework Directive. Inundation tests provide an indication that bank sediments have the potential to contribute dissolved Pb to surface water.

Conclusions

The determination of Pb in the interstitial water and in the inundation water, taken with water Pb mass balance and sediment Pb distribution maps at the catchment scale, implicate the contaminated sediments as a large Pb supply to surface water. Assessment of these diffuse contaminant sources is critical for the successful management of mining-impacted catchments.  相似文献   

17.

Purpose

Hydrosedimentological modeling is a tool that can be used to understand better important processes occurring at the catchment scale, such as runoff and sediment yield. The aim of this study was to use the Limburg Soil Erosion Model (LISEM) to describe the runoff and sediment yield during rainfall–runoff events in a small rural catchment in southern Brazil.

Materials and methods

The study was conducted in the Lajeado Ferreira Creek catchment (drainage area of 1.19 km2) where intense land use has caused a negative impact on water resources. Thirteen rainfall–runoff events that occurred in 2010 and 2011, including high-magnitude events, were used to model hydrosedimentological processes.

Results and discussion

Results

from the calibration and validation stages indicate that the model had a good performance when representing the hydrograph, including events with greater complexity. The use of a second soil layer in the model increased its efficiency, which is in accordance with the importance of subsurface flow in this catchment and its sensitivity to the physical properties of the soil, which are essential for controlling hydrosedimentological processes at the catchment scale. The simulation of sediment yield was overestimated by the model, constrained by the lack of sensitivity of the model to soil cohesion and the stability of soil aggregates. During the model calibration stage, these parameters had values different from those measured in the field.

Conclusions

The LISEM model performed well in representing runoff for events of different magnitudes. The discretization of the physical–hydrologic properties in the soil profile enabled the evaluation of the effect of subsurface impediment layers on water infiltration and runoff. The simulation was less accurate for suspended sediment concentration than for runoff. This indicates the need for further studies to either identify other factors controlling erosion and sediment yield that have not been identified by the model, or identify if the representation of the physical parameters is inadequate, especially the values of soil cohesion and aggregate stability.  相似文献   

18.

Purpose

Dominant discharges and associated sediment dynamics of the River Isábena, a 445-km2 catchment in the central Pyrenees of Spain that is punctuated by badlands, are analysed.

Materials and methods

Calculations of suspended sediment loads are based on continuous records of discharge and turbidity obtained at the basin outlet for the period 2005–2010.

Results and discussion

Dominant discharges for sediment load (i.e. effective discharge) present a bimodal distribution, with one peak falling in the range of low flows and the other associated to less frequent but higher magnitude floods (i.e. bankfull). The highly suspended sediment availability in the badlands, together with the high connectivity between the badlands and the stream network and the important in-channel fine sediment storage, causes both large and small events to remobilize fines. Baseflows, despite their low competence, generate resuspension and massive sediment loads. Thus, effective discharge (i.e. the discharge which transports most of the sediment) is not solely associated with bankfull (i.e. the discharge that dominates channel form), but to a wider range of discharges. Consequently, this river channel is not specifically adjusted to convey most of the sediment load during high floods, as in many other rivers, but instead large volumes of sediment are transferred downstream at an almost constant rate.

Conclusions

Results suggest that dominant discharge may play a lesser role in terms of (suspended) sediment load in non-supply-limited fluvial systems and/or in rivers that permanently work close to, or at, full transport capacity, as is the case of the Isábena.  相似文献   

19.

Purpose

Almost 20 nuclear reactors are situated along the Rh?ne valley, representing Europe??s largest concentration of nuclear power plants. The fate of suspended sediments and natural and artificial particle-bound radionuclides in relation to extreme hydrological events was assessed at the lower course of the Rh?ne River, which provides the main source of water and sediment inputs to the northwestern Mediterranean Sea.

Materials and methods

We sampled water at a high frequency over the period 2001?C2008 and measured suspended particulate matter (SPM) loads and particle-bound natural and artificial radionuclide concentrations at the SORA observatory station in Arles, France. We monitored various hydrological events (either natural or anthropogenic origin) and characterize their influence on concentrations and fluxes.

Results and discussion

The relationship between SPM concentration and the very wide range of water discharges did not differ significantly from previous periods, indicating no significant shift in the average sediment delivery over the last 20?years. Unexpected hydrological events of anthropogenic origin, in particular those associated with flushing of reservoirs that are generally not captured by sampling strategies, were recorded and were shown to transfer significant additional sediment and associated contaminants towards the marine environment. Concentrations of anthropogenic radionuclides associated with sediment (i.e., 137Cs, 60Co, 54Mn, 110mAg, and Pu isotopes) varied over two to three orders of magnitude during periods of low and moderate flow due to variations in the liquid release from nuclear facilities. Except for Pu isotopes, the concentrations of the various particle-bound radionuclides generally showed a decreasing trend with increasing discharge, revealing the geochemical or anthropogenic background values, and providing a useful flood fingerprint for this large fluvial system before its entry into the marine environment.

Conclusions

Our approach produced key data on the level and fate of suspended solids and radionuclide concentrations during flood events occurring in a large river system that could be contaminated by chronic or accidental radioactive releases. These results are of fundamental importance for further interpretations of sediment dynamics at the river mouth.  相似文献   

20.
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