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1.
通过盆栽试验方法,选择经济作物甜菜和牧草类黑麦草、苏丹草、香根草为供试植物,研究了甜菜与3种牧草分别间作及各自单作对多环芳烃(PAHs)菲、荧蒽、芘和苯并[a]芘污染土壤修复作用。结果显示:经6个月连续两茬种植试验后,所有种植植物的处理中土壤PAHs的去除率均高于无植物种植组,间作种植土壤PAHs的去除率高于单作,黑麦草、苏丹草、香根草与甜菜间作对土壤PAHs的去除率分别达到84.85%、79.96%、84.11%;在土壤污染条件下,间作模式更有利于甜菜生长;种植植物增强了土壤中多酚氧化酶和过氧化氢酶的活性,间作模式下二者活性高于单作4.37%~43.07%,过氧化氢酶较多酚氧化酶对PAHs土壤污染更敏感,可作为关键酶用于评价土壤PAHs污染状况。在不影响农业生产的前提下,修复植物牧草和经济作物甜菜间作种植模式显著提高了土壤PAHs的降解率。  相似文献   

2.
为明确微生物菌剂改善大蒜产地环境、提升产量品质的效果,利用常规施肥结合解淀粉芽孢杆菌W48发酵液进行大蒜田土壤处理,测定大蒜产量和品质相关指标,监测土壤理化性质及生物转化相关酶活性变化,定量分析菌剂处理后土壤和大蒜中邻苯二甲酸酯类塑化剂(PAEs)含量差异。结果表明,W48菌株具有分泌吲哚乙酸的能力,同时具备溶磷和产铁载体的潜力。施用W48微生物菌剂显著增加了植物根际土壤有机质、碱解氮、有效磷和速效钾含量,改善根际区域营养环境,提高了土壤碱性磷酸酶、蔗糖酶和脲酶等生物转化相关酶活性,提高了土壤氮、磷元素利用效率;与对照相比,微生物菌剂处理的小区大蒜增产10%,可溶性糖和维生素C含量等品质指标均有提高,其中可溶性糖显著增加了30%;邻苯二甲酸二正丁酯(DBP)和邻苯二甲酸二(2-乙基)己酯(DEHP)是土壤和大蒜中PAEs的主要检出类型,土壤中的平均浓度分别达到1874.05和337.12μg/kg,大蒜中几种PAEs残留量普遍较高,DBP最高为666.57μg/kg,其次为邻苯二甲酸二异丁酯(DIBP)409.93μg/kg和邻苯二甲酸丁苄酯(BBP)433.65μg/kg。菌剂对PA...  相似文献   

3.
金桔园土壤及金桔中酞酸酯污染特征分析   总被引:1,自引:0,他引:1  
对金桔园土壤及金桔中酞酸酯污染特征进行了分析,结果表明:调查的6种酞酸酯,5个土壤监测点DMP、DEP、DOP、BBP都未检出;DBP、DEHP全部都有检出,各土壤监测点中DBP浓度值均比DEHP浓度值高。3个金桔样中DMP、DOP、BBP都未检出;DEHP、DBP、DEP全部都有检出,PAEs浓度值都遵循DEHP>DBP>DEP的规律。金桔果实对PAEs的吸收积累途径主要是通过果实外表皮直接吸收塑料大棚中的PAEs蒸汽。  相似文献   

4.
以不同浓度DBP和DEHP处理的土壤对青菜、菠菜、莴苣和萝卜进行盆栽实验,采用加速溶剂萃取,Qu ECh ERS方法和硅烷衍生化对土壤和蔬菜样品进行前处理,结合气相色谱-串联质谱(GC-MS/MS)检测技术,分析了4种蔬菜中DBP、DEHP及其单酯代谢物MBP、MEHP从土壤中吸收的残留量分布规律和富集系数。结果表明,生长在高、低两个不同浓度DBP和DEHP土壤中的4种蔬菜都有DBP、DEHP及其代谢物MBP和MEHP的检出。萝卜中DBP和DEHP残留总量(Σ2PAEs)及其代谢物残留总量均明显高于其他3种蔬菜。4种蔬菜对土壤中的DEHP的生物富集因子BCF值都大于1,有明显的富集效应;而对于土壤中DBP有富集效应的则只有萝卜,其他3种蔬菜对DBP的BCF值都远小于1。相关研究结果表明,土壤中的DBP、DEHP能被蔬菜产品吸收富集,并且在体内代谢出毒性比母体更高的单酯产物。  相似文献   

5.
选用黄棕壤和红壤,用土壤老化和上海青(Brassica campestris)盆栽试验研究了邻苯二甲酸二正丁酯(Di-butyl Phthalate,DBP)和邻苯二甲酸二异辛酯(D(i2-ethylhexyl)Phthalate,DEHP)在土壤-植物系统中的分布规律。土壤老化试验表明,DBP和DEHP在土壤中的吸附量随着老化时间的增加,呈现开始(0-10 d)老化速率较快,而后(10-30 d)老化速率减小并且老化总量趋于稳定的趋势。盆栽试验结果表明,在红壤上植物体内DBP/DEHP含量(DBP:0.576-2.750 mg.kg-1;DEHP:9.369-33.256 mg.kg-1)与土壤污染浓度呈正相关,生物量与土壤污染浓度呈负相关;而在黄棕壤上,上海青的生物量并不随着土壤DBP/DEHP的添加量的升高而变化,植物体内DBP/DEHP的含量(DBP:0.212-0.401 mg.kg-1;DEHP:0.421-0.490 mg.kg-1)远低于红壤的相同污染浓度处理。在黄棕壤上,上海青对DBP/DEHP的BCF值介于0.061-1.041之间;而在红壤上,BCF值均大于1.0(介于1.175-15.695之间),具有一定的生物富集作用。通过试验还估算了红壤上DBP/DEHP的临界浓度为6.932-11.718 mg.kg-1,可为建立生态效应预警指标提供参考。  相似文献   

6.
菜心对邻苯二甲酸酯(PAEs)吸收途径的初步研究   总被引:16,自引:2,他引:16  
采用玻璃室处理和污染土壤覆盖原土壤来控制PAEs来源进行盆栽试验,应用GC/MS联机检测技术初步研究了菜心对PAEs的吸收途径。结果表明:污染土壤处理与污染土壤上覆盖原土壤处理相比,前者菜心茎叶中DBP和DEHP的含量均高于后者,但相差不大,表明菜心茎叶可以吸收污染土壤中挥发出来的DBP和DEHP,而根系吸收运移是菜心茎叶中DBP和DEHP的主要来源途径。玻璃室处理增加了菜心茎叶和根系中DBP的含量,而对DEHP的影响趋势不明显。DBP与DEHP相比,前者更易被菜心根系吸收并向地上部(茎叶)运移,后者主要滞留在根部。  相似文献   

7.
以大豆、黑麦草和南瓜为材料,运用盆栽实验,通过3种植物的单作和间作对多氯联苯污染土壤的根际修复效应进行了研究。结果表明,植物不同种植方式均对根际土壤中PCB浓度的降解有促进作用,其中植物单作的去除率比CK提高了10.4%~17.0%,植物间作的去除率比CK提高18.4%~23.9%。南瓜-大豆体系中的大豆根的蓄积浓度显著差异高于其他处理,而与大豆南瓜间作方式下黑麦草根蓄积浓度均比其单作显著提高,大豆-南瓜和南瓜-黑麦草间作系统中的大豆和黑麦草根中PCB蓄积浓度也显著提高(P〈0.05)。各处理间根际土壤的pH、Eh、电导率的差异性规律性不大。相关分析结果表明,根际土壤PCB去除率与植物吸收量呈显著正相关,而与pH、Eh和电导率没有达到显著相关。  相似文献   

8.
湖州地区土壤邻苯二甲酸酯空间分布现状特征分析   总被引:1,自引:0,他引:1  
采用气相色谱-质谱联用方法,对湖州地区表层土壤样品中6种邻苯二甲酸酯类化合物进行了联合测定。结果表明,邻苯二甲酸二(2-乙基己基)酯(DEHP)是湖州地区土壤中主要的邻苯二甲酸酯类污染物;6种PAEs的总含量在nd(未检出)~1.1009mg·kg-1之间;与美国土壤中PAEs标准限值相比,有个别区域的邻苯二甲酸二丁酯(DnBP)超标;湖州地区土壤中PAEs整体污染状况较轻。  相似文献   

9.
玉米苜蓿间作的蓄水保土效益试验研究   总被引:4,自引:0,他引:4  
为了在种植作物的同时减少水土流失,采用玉米苜蓿间作的种植模式,研究其蓄水保土效益。试验对玉米苜蓿间作与单作玉米的土壤含水量,径流量以及产沙量进行观测,进而研究两者的蓄水保土效益。结果表明:玉米苜蓿间作地的土壤含水量大于玉米单作地的土壤含水量;玉米苜蓿间作的径流量和产沙量均小于玉米单作,说明了玉米苜蓿能够有效地减少径流的冲刷侵蚀,具有良好的拦沙性能;经计算得出玉米苜蓿间作的蓄水效益为87%,保土效益为98%,表明玉米苜蓿间作的蓄水保土效益显著。  相似文献   

10.
北京市东南郊灌区土壤和农产品酞酸酯污染风险评估   总被引:4,自引:0,他引:4  
为明确北京市东南郊典型灌区土壤和作物酞酸酯PAEs含量和污染水平,2015年利用气象色谱-质谱仪检测了该灌区31个表层土壤样品和38个作物样品的6种优控PAEs含量.研究结果表明灌区表层土壤PAEs质量分数为1.8~12.2 mg/kg,均值5.1 mg/kg.与国内外相比,该研究中土壤PAEs含量处于较高水平.土壤中邻苯二甲酸正二丁酯(DnBP)和邻苯二甲酸二(2-乙基己基)酯(DEHP)含量均值分别占PAEs总量的60.4%和35.9%.土壤样品邻苯二甲酸二甲酯(DMP)和DnBP含量均超美国土壤PAEs控制标准,但总体上未超过美国土壤PAEs治理标准.冬小麦籽粒、夏玉米籽粒和果蔬可食用部位PAEs质量分数分别为2.34~3.66、1.76~3.15和2.26~3.76 mg/kg;与其他研究成果相比,该研究区农产品PAEs含量处于中等水平.不同污灌历史年限区域土壤和粮食作物籽粒PAEs含量均没有显著差异.冬小麦籽粒、夏玉米籽粒和果蔬中DEHP和DnBP含量分别占总量的50.3%和30.5%、45.1%和50.2%、47.16%~63.3%和31.96%~46.36%.农产品PAEs总量及各组分含量均低于欧洲的建议标准值.粮食作物籽粒中PAEs和DnBP含量与土壤中相应含量呈显著正相关,Pearson相关系数(r)分别为0.74~0.87和0.91~0.92.该研究中农作物对PAEs的迁移系数为0.24~1.65.儿童和成人PAEs致癌风险分别为1.34×10-5和3.87x10-5,非致癌指数分别为9.44x 10-1和3.83×10-1,均在可接受范围内;通过口-作物暴露对PAEs 2种风险贡献均最大,DEHP对人体2种风险贡献最大.  相似文献   

11.
Phthalate esters(PAEs) are extensively applied in industry, and they migrate to environment during the process of production,employ, and treatment and are difficult to be degraded in nature. However, some microorganisms could use them as the carbon source to growth. In this study, an Acinetobacter sp. strain LMB-5, capable of utilizing PAEs, was isolated from a vegetable greenhouse soil.The degradation capability of strain LMB-5 was also investigated by incubation in mineral salt medium containing different PAEs,dimethyl phthalate(DMP), diethyl phthalate(DEP), di-n-butyl phthalate(DBP), and di-(2-ethylhexyl) phthalate(DEHP). The strain could grow well with DMP, DEP, DBP, and DEHP. When the concentration of DBP increased from 100 to 400 mg L~(-1), the half-life extended from 9.5 to 15.5 h. In the concentration range of DBP, the degradation ability of strain LMB-5 could be described by first-order kinetics. During the biodegradation of DBP, three intermediates, 1,2-benzenedicarboxylic acid,butyl methyl ester, DMP,and phthalic acid(PA) were detected, and the proposed pathway of DBP was identified. By analysis of bioinformatics, one esterase was cloned from the genome of LMB-5 and expressed in Escherichia coli. It displayed an ability to break the ester bonds of DBP. The enzyme exhibited maximal activity at pH 7.0 and 40℃ with DBP as the substrate. It was activated by Cu~(2+) and Fe~(3+) and had a high activity in the presence of low concentrations of methanol or dimethylsulfoxide(each 10%, volume:volume). The Acinetobacter sp. strain LMB-5 may make a contribution to the remediation of soils polluted by PAEs in the future.  相似文献   

12.
【目的】分析间作修复对镉(Cd)污染农田玉米Cd含量影响,旨在为实现污染农田边生产边修复提供基础支撑。【方法】本研究以“玉米”、“Cd”、“间作”为关键词,在“中国知网”和“Web of Science”数据库检索2006—2020年期间发表的文献,筛选出符合要求的文献33篇,获得数据770组。以玉米单作为对照,利用整合分析(meta-analysis)方法揭示间作修复对玉米Cd含量影响,明确间作植物种类、玉米品种、土壤性质和栽培措施等因素的综合效应。【结果】与单作玉米相比,大田间作修复能显著降低玉米籽粒、茎叶和根Cd含量,尤其对籽粒Cd抑制作用最显著。蜈蚣草+籽粒苋、蜈蚣草、籽粒苋和龙葵等间作植物对玉米籽粒Cd含量有显著抑制作用;东单、海禾28和绿玉269等玉米品种籽粒Cd含量也显著受间作修复抑制。在弱酸性或中性土壤上,间作修复对玉米籽粒Cd的抑制作用增强;无论是安全利用类还是严格管控类农田,间作修复均能显著降低玉米籽粒Cd含量;间作行距对玉米籽粒和茎叶Cd含量影响不显著,但0~30 cm行距显著降低根Cd含量。盆栽间作修复涉及到的间作植物以及玉米品种较多,Meta分析结果表明,盆栽...  相似文献   

13.

Purpose

We investigated the effect of growth strategy (i.e., single or mixed plant types) of two emergent plants (i.e., Phragmites australis and Typha orientalis) on the distribution of phthalic acid esters (PAEs) and their monoester metabolites (PAMs) in the sediments and roots in two adjacent shallow lakes in Tianjin, China, as well as the removal of PAEs from the sediments.

Materials and methods

Dibutyl phthalate (DBP), di-2-ethylhexyl phthalate (DEHP), and their PAMs were measured in sediments and roots sampled on 18th May 2010. PAE-degrading bacteria and phospholipid fatty acid (PLFA) of the sediment samples were also analyzed.

Results and discussion

The results showed that DBP, DEHP, and their PAMs were detected in nearly all of the samples, and the PAE concentrations were 1 to 2 orders of magnitude higher than those of their corresponding monoester metabolites. The PAE distribution patterns in sediments from the two lakes were different and influenced by plant growth strategy. Phytoavailability of PAEs was also affected by plant growth strategy.

Conclusions

Compared with the non-rhizosphere sediments, the total organic carbon-normalized PAE concentration in the rhizosphere sediments decreased in the presence of the emergent plants. The PAE removal from the rhizosphere sediments was related not only to plant species but also to growth strategy, which was consistent with the findings of PLFA. The enhancement of PAE biodegradation in the rhizosphere was mainly the result of changes in the microbial community structure for different plant species and in microbial biomass for the same plant species.  相似文献   

14.
盆栽试验条件下,通过外源添加DBP/DEHP制成0,20,50,100,200 mg/kg的浓度梯度,来研究PAEs对烟草生长的影响及其在土壤-烟草系统的累积特征。结果表明:外源DBP/DEHP的添加对烟草地上部生物量和茎粗无显著影响,烟草株高随外源DBP/DEHP浓度的增加呈现不同的变化趋势,其中黄棕壤烟草株高显著降低,红壤的显著增加,而黄壤的无变化;黄壤根系活力随外源DBP/DEHP浓度先增高后降低,而黄棕壤和红壤的无显著变化。DBP/DEHP浓度对部分烟草抗氧化酶活性有显著影响,而对土壤的脱氢酶和和脲酶活性基本无影响。随外源PAEs浓度的增加,土壤中DBP/DEHP含量均呈现上升的趋势,以黄棕壤DBP含量增加幅度最大,添加200 mg/kg DBP时是CK(外源不添加DBP/DEHP)的3.56倍;黄棕壤和红壤DEHP浓度大幅增加,黄棕壤和红壤添加200 mg/kg DEHP时分别是CK的27.47,27.34倍。相比于CK大多数烟叶中和根系中DBP/DEHP有不同程度的提升。随外源DBP/DEHP浓度的增加,会在一定程度上促进土壤和烟叶DBP/DEHP的积累。  相似文献   

15.
选择了经济相对发达的珠江三角洲城市群中的典型中小城市的菜地和果园土壤进行调查取样,对16种PAEs(邻 苯二甲酸酯)化合物进行了检测,以研究其分布特征,并初步探讨了本区域的PAEs的污染控制问题。结果表明,在珠三角城市中,东莞土壤的PAEs含量最高,各地土壤中的PAEs平均含量依次为东莞〉深圳(珠海)〉中山(惠州);从珠三角城市菜地和果园的平均PAEs分布来看,东莞和深圳的菜地PAEs明显高于果园;珠海、中山和惠州菜地的平均PAEs与果园基本持平。16种PAEs类化合物在珠江三角洲不同城市的分布各异,东莞市果园和菜地土壤中有11种PAEs含量是采样的5个城市中最高的,表明东莞市土壤受到PAEs污染相对严重,并且值得关注的是东莞土壤中的HEP含量要远远高于其他PAEs化合物。虽然与国内外其他城市土壤相比,所取样调查的珠江三角洲城市土壤中的PAEs含量相对不高,但与美国土壤PAEs控制标准相比,珠三角城市果园和菜地土壤的PAEs主要表现为DEP和DnBP超标,这两类PAEs化合物应该成为重点的污染控制对象。  相似文献   

16.
Single phytotoxicity of two representative phthalate esters (PAEs), di-n-butyl phthalate (DnBP) and bis(2-ethylhexyl) phthalate (DEHP), was tested in mung bean (Vigna radiata) seedlings germinated for 72 h in soils spiked with varying concentrations (0-500 mg kg-1 soil) of DnBP or DEHP. PAEs added at up to 500 mg kg-1 soil exerted no significant effect on germination but both pollutants significantly inhibited root elongation (P 〈 0.01); DEHP inhibited shoot elongation (P 〈 0.01) and DnBP depressed biomass on a fresh weight basis (P 〈 0.05). Seedling shoot and root malondialdehyde (MDA) Contents tended to be stimulated by DnBP but inhibited by DEHP. However, increases in superoxide dismutase, peroxidase, ascorbate peroxidase and polyphenol oxidase activities, as well as glutathione (GSH) content, were induced at higher concentrations (e.g., 20 mg kg-1) of both compounds. Accumulation of proline in both roots and shoots and the storage compounds, such as free amino acids and total soluble sugars, in whole plant was induced under the stress exerted by both PAEs. The general responses of mung bean seedlings indicated higher toxicity of DnBP than DEHP on primary growth, during which root elongation was a more responsive index. MDA and GSH were more sensitive parameters in the roots than in the shoots and they might be recommended as physiologically sensitive parameters to assess the toxicity of PAE compounds in soils in future long-term studies.  相似文献   

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