共查询到20条相似文献，搜索用时 250 毫秒
1.
van der Wiel WG De Franceschi S Fujisawa T Elzerman JM Tarucha S Kouwenhoven LP 《Science (New York, N.Y.)》2000,289(5487):2105-2108
We observe a strong Kondo effect in a semiconductor quantum dot when a small magnetic field is applied. The Coulomb blockade for electron tunneling is overcome completely by the Kondo effect, and the conductance reaches the unitary limit value. We compare the experimental Kondo temperature with the theoretical predictions for the spin- 12 Anderson impurity model. Excellent agreement is found throughout the Kondo regime. Phase coherence is preserved when a Kondo quantum dot is included in one of the arms of an Aharonov-Bohm ring structure, and the phase behavior differs from previous results on a non-Kondo dot. 相似文献
2.
Zhao A Li Q Chen L Xiang H Wang W Pan S Wang B Xiao X Yang J Hou JG Zhu Q 《Science (New York, N.Y.)》2005,309(5740):1542-1544
We report that the Kondo effect exerted by a magnetic ion depends on its chemical environment. A cobalt phthalocyanine molecule adsorbed on an Au111 surface exhibited no Kondo effect. Cutting away eight hydrogen atoms from the molecule with voltage pulses from a scanning tunneling microscope tip allowed the four orbitals of this molecule to chemically bond to the gold substrate. The localized spin was recovered in this artificial molecular structure, and a clear Kondo resonance was observed near the Fermi surface. We attribute the high Kondo temperature (more than 200 kelvin) to the small on-site Coulomb repulsion and the large half-width of the hybridized d-level. 相似文献
3.
We measured the phase evolution of electrons as they traverse a quantum dot (QD) formed in a two-dimensional electron gas that serves as a localized spin. The traversal phase, determined by embedding the QD in a double path electron interferometer and measuring the quantum interference of the electron wave functions manifested by conductance oscillation as a function of a weak magnetic field, evolved by pi radians, a range twice as large as theoretically predicted. As the correlation weakened, a gradual transition to the familiar phase evolution of a QD was observed. The specific phase evolution observed is highly sensitive to the onset of Kondo correlation, possibly serving as an alternative fingerprint of the Kondo effect. 相似文献
4.
Double quantum dots provide an ideal model system for studying interactions between localized impurity spins. We report on the transport properties of a series-coupled double quantum dot as electrons are added one by one onto the dots. When the many-body molecular states are formed, we observe a splitting of the Kondo resonance peak in the differential conductance. This splitting reflects the energy difference between the bonding and antibonding states formed by the coherent superposition of the Kondo states of each dot. The occurrence of the Kondo resonance and its magnetic field dependence agree with a simple interpretation of the spin status of a double quantum dot. 相似文献
5.
Craig NJ Taylor JM Lester EA Marcus CM Hanson MP Gossard AC 《Science (New York, N.Y.)》2004,304(5670):565-567
The effective interaction between magnetic impurities in metals that can lead to various magnetic ground states often competes with a tendency for electrons near impurities to screen the local moment (known as the Kondo effect). The simplest system exhibiting the richness of this competition, the two-impurity Kondo system, was realized experimentally in the form of two quantum dots coupled through an open conducting region. We demonstrate nonlocal spin control by suppressing and splitting Kondo resonances in one quantum dot by changing the electron number and coupling of the other dot. The results suggest an approach to nonlocal spin control that may be relevant to quantum information processing. 相似文献
6.
An experimental method based on the Landau-Zener model was developed to measure very small tunnel splittings in molecular clusters of eight iron atoms, which at low temperature behave like a nanomagnet with a spin ground state of S = 10. The observed oscillations of the tunnel splittings as a function of the magnetic field applied along the hard anisotropy axis are due to topological quantum interference of two tunnel paths of opposite windings. Transitions between quantum numbers M = -S and (S - n), with n even or odd, revealed a parity effect that is analogous to the suppression of tunneling predicted for half-integer spins. This observation is direct evidence of the topological part of the quantum spin phase (Berry phase) in a magnetic system. 相似文献
7.
Single-walled carbon nanotubes are ideal systems for investigating fundamental properties and applications of one-dimensional electronic systems. The interaction of magnetic impurities with electrons confined in one dimension has been studied by spatially resolving the local electronic density of states of small cobalt clusters on metallic single-walled nanotubes with a low-temperature scanning tunneling microscope. Spectroscopic measurements performed on and near these clusters exhibit a narrow peak near the Fermi level that has been identified as a Kondo resonance. Using the scanning tunneling microscope to fabricate ultrasmall magnetic nanostructures consisting of small cobalt clusters on short nanotube pieces, spectroscopic studies of this quantum box structure exhibited features characteristic of the bulk Kondo resonance, but also new features due to finite size. 相似文献
8.
Pasupathy AN Bialczak RC Martinek J Grose JE Donev LA McEuen PL Ralph DC 《Science (New York, N.Y.)》2004,306(5693):86-89
We measured Kondo-assisted tunneling via C60 molecules in contact with ferromagnetic nickel electrodes. Kondo correlations persisted despite the presence of ferromagnetism, but the Kondo peak in the differential conductance was split by an amount that decreased (even to zero) as the moments in the two electrodes were turned from parallel to antiparallel alignment. The splitting is too large to be explained by a local magnetic field. However, the voltage, temperature, and magnetic field dependence of the signals agree with predictions for an exchange splitting of the Kondo resonance. The Kondo effect leads to negative values of magnetoresistance, with magnitudes much larger than the Julliere estimate. 相似文献
9.
We used a scanning tunneling microscope to probe the interactions between spins in individual atomic-scale magnetic structures. Linear chains of 1 to 10 manganese atoms were assembled one atom at a time on a thin insulating layer, and the spin excitation spectra of these structures were measured with inelastic electron tunneling spectroscopy. We observed excitations of the coupled atomic spins that can change both the total spin and its orientation. Comparison with a model spin-interaction Hamiltonian yielded the collective spin configuration and the strength of the coupling between the atomic spins. 相似文献
10.
A tunable kondo effect in quantum dots 总被引：1，自引：0，他引：1
A tunable Kondo effect has been realized in small quantum dots. A dot can be switched from a Kondo system to a non-Kondo system as the number of electrons on the dot is changed from odd to even. The Kondo temperature can be tuned by means of a gate voltage as a single-particle energy state nears the Fermi energy. Measurements of the temperature and magnetic field dependence of a Coulomb-blockaded dot show good agreement with predictions of both equilibrium and nonequilibrium Kondo effects. 相似文献
11.
Intermolecular electron transfer by quantum mechanical tunneling 总被引：1，自引：0，他引：1
Miller JR 《Science (New York, N.Y.)》1975,189(4198):221-222
The transfer of electrons from one molecule to another by quantum mechanical tunneling has recently been implicated in biological electron transport. This report describes observations of electron transfer between aromatic molecules in a rigid matrix, in which electrons apparently tunnel through tens of angstroms of inert solvent. The kinetics tend to confirm the tunneling process, which is likely to be an important means of electron transfer when diffusion is blocked by steric factors or immobilization of the reactants. 相似文献
12.
Single spins in solid-state systems are often considered prime candidates for the storage of quantum information, and their interaction with the environment the main limiting factor for the realization of such schemes. The lifetime of an excited spin state is a sensitive measure of this interaction, but extending the spatial resolution of spin relaxation measurements to the atomic scale has been a challenge. We show how a scanning tunneling microscope can measure electron spin relaxation times of individual atoms adsorbed on a surface using an all-electronic pump-probe measurement scheme. The spin relaxation times of individual Fe-Cu dimers were found to vary between 50 and 250 nanoseconds. Our method can in principle be generalized to monitor the temporal evolution of other dynamical systems. 相似文献
13.
Taguchi Y Oohara Y Yoshizawa H Nagaosa N Tokura Y 《Science (New York, N.Y.)》2001,291(5513):2573-2576
An electron hopping on non-coplanar spin sites with spin chirality obtains a complex phase factor (Berry phase) in its quantum mechanical amplitude that acts as an internal magnetic field, and is predicted to manifest itself in the Hall effect when it is not cancelled. The present combined work of transport measurement, neutron scattering, and theoretical calculation provides evidence that the gigantic anomalous Hall effect observed in Nd2Mo2O7, a pyrochlore ferromagnet with geometrically frustrated lattice structure, is mostly due to the spin chirality and the associated Berry phase originating from the Mo spin tilting. 相似文献
14.
Delft J 《Science (New York, N.Y.)》2000,289(5487):2064-2065
Advances in mesoscopic physics are enabling fundamental properties of solids to be studied at an unprecedented level of detail. In his Perspective, von Delft highlights the study by van der Wiel et al., who have demonstrated almost complete screening of the local spin of a quantum dot. This behavior mirrors the well-known Kondo effect for magnetic impurities in metals. Because they are tunable, quantum dots allow detailed tests of models for the Kondo effect, but experiments are ahead of theory at this time. 相似文献
15.
We measure the differential conductance of a single-electron transistor (SET) irradiated with microwaves. The spin-entangled many-electron Kondo state produces a zero-bias peak in the dc differential conductance if the quantum dot in the SET contains an unpaired electron. When the photon energy hf is comparable to the energy width of the Kondo peak and to e (the charge on the electron) times the microwave voltage across the dot, satellites appear in the differential conductance shifted in voltage by +/-hf/e from the zero-bias resonance. We also observe an overall suppression of the Kondo features with increasing microwave voltage. 相似文献
16.
Control of magnetism on the atomic scale is becoming essential as data storage devices are miniaturized. We show that antiferromagnetic nanostructures, composed of just a few Fe atoms on a surface, exhibit two magnetic states, the Néel states, that are stable for hours at low temperature. For the smallest structures, we observed transitions between Néel states due to quantum tunneling of magnetization. We sensed the magnetic states of the designed structures using spin-polarized tunneling and switched between them electrically with nanosecond speed. Tailoring the properties of neighboring antiferromagnetic nanostructures enables a low-temperature demonstration of dense nonvolatile storage of information. 相似文献
17.
The miniaturization of magnetic devices toward the limit of single atoms calls for appropriate tools to study their magnetic properties. We demonstrate the ability to measure magnetization curves of individual magnetic atoms adsorbed on a nonmagnetic metallic substrate with use of a scanning tunneling microscope with a spin-polarized tip. We can map out low-energy magnetic interactions on the atomic scale as evidenced by the oscillating indirect exchange between a Co adatom and a nanowire on Pt(111). These results are important for the understanding of variations that are found in the magnetic properties of apparently identical adatoms because of different local environments. 相似文献
18.
Dutt MV Childress L Jiang L Togan E Maze J Jelezko F Zibrov AS Hemmer PR Lukin MD 《Science (New York, N.Y.)》2007,316(5829):1312-1316
The key challenge in experimental quantum information science is to identify isolated quantum mechanical systems with long coherence times that can be manipulated and coupled together in a scalable fashion. We describe the coherent manipulation of an individual electron spin and nearby individual nuclear spins to create a controllable quantum register. Using optical and microwave radiation to control an electron spin associated with the nitrogen vacancy (NV) color center in diamond, we demonstrated robust initialization of electron and nuclear spin quantum bits (qubits) and transfer of arbitrary quantum states between them at room temperature. Moreover, nuclear spin qubits could be well isolated from the electron spin, even during optical polarization and measurement of the electronic state. Finally, coherent interactions between individual nuclear spin qubits were observed and their excellent coherence properties were demonstrated. These registers can be used as a basis for scalable, optically coupled quantum information systems. 相似文献
19.
Quantum tunneling, the passage of a microscopic system from one state to another by way of a classically forbidden path, is theoretically possible in the macroscopic world. One can now make direct observations of such macroscopic quantum tunneling in very small magnetic structures. This is possible because of significant advances both in the ability to obtain magnetic systems of almost any desirable size, shape, and composition and in the development of superconducting instrumentation for the detection of extremely weak magnetic signals. As an example, measurements on magnetic horse spleen ferritin proteins with the predictions of quantum tunneling theory are discussed and shown. 相似文献
20.
Silicon microstructures only a few hundred atoms wide can be fabricated and used to study electron transport in narrow channels. Spatially localized voltage probes as close together as 0.1 micrometer can be used to investigate a variety of physical phenomena, including velocity saturation due to phonon emission, the local potentials caused by scattering from a single trapped electron, and quantum tunneling or hopping among very few electron states. 相似文献