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1.
Abstract

Biofortification of soybean grains with lithium (Li) is a strategy to improve a food with high social acceptance, in order to promote health benefits. The aim of this work was to evaluate the development of plants and the production of biofortified soybeans with two Li sources. The experiment was conducted in a completely randomized design with five replicates. Ten treatments were obtained in a 2x5 factorial scheme, comprising two sources of Li (LiOH - Li hydroxide and Li2SO4 - Li sulfate) and five doses (0, 30, 60, 90 and 120?mg kg?1) in stages V4 and R1. The supply of Li promoted significant effects (p?≤?0.05) on the morphology, yield components and nutritional status of soybean plants. The highest grain yield was obtained with the use of Li2SO4 at the estimated dose of 45.7?mg kg?1. The plants accumulated Li between 8.00 and 11.20?mg kg ?1, respectively, with the use of Li2SO4 and LiOH. In the grains, the highest concentrations of Li were obtained with the application of 120?mg kg?1. Li2SO4 and LiOH are good sources for biofortification of soybean grains.  相似文献   

2.
Information related to phosphate fertilization and coated phosphate fertilizer in lettuce (Lactuca sativa L.) is scarce. Thus, this study was carried out to evaluate the agronomic efficiency, production, and nutritional characteristics of coated monoammonium phosphate (MAP) in two subsequent crops with lettuce cv. Solaris. The experimental design was completely randomized (2 x 5 factorial experiment): two sources of phosphorus (P) (MAP and coated MAP), five applications (0; 75; 150; 300; and 600 mg phosphorus pentoxide (P2O5) kg?1) with four replications. In the first crop, there was a greater accumulation of P in plants shoot with the application of coated MAP until 150 mg P2O5 kg?1 dose, surpassed by MAP after this dose. On the second crop, fresh mass and the accumulation of P in the leaves were higher than the uncoated MAP. In both crops, the agronomic efficiency of P fertilization decreased with increase in the amount of phosphorus applied in lettuce cultivation.  相似文献   

3.
This study was conducted to evaluate the roles of glycine betaine (GB) in mitigating deleterious effect of salt stress on lettuce. Lettuce plants were subjected to two salinity (0 and 100 mmol l?1 NaCl) and four GB levels (0, 5, 10, 25 mmol l?1). Salinity resulted in a remarkable decrease in growth parameters, relative leaf water content and stomatal conductance. Plants subjected to salt stress exhibited an increase in membrane permeability (MP), lipid peroxidation (MDA), leaf chlorophyll reading value, H2O2 and sugar content. Exogenous foliar applications of GB reduced MP, MDA and H2O2 content in salt-stressed lettuce plants. Salt stress increased Na and generally decreased other nutrient elements. GB reduced Na accumulation, but significantly increased other element contents under salinity conditions. The study showed that gibberellic acid (GA) and salicylic acid (SA) content in salt-stressed plants were lower than those of nonstressed plants. However, salinity conditions generally increased the abscisic acid content. GB treatments elevated the concentrations of GA, SA and indole acetic acid (IAA) at especially 10 and 25 mmol l?1 GB under salt stress conditions. It could be concluded that exogenous GB applications could ameliorate the harmful effects of salt stress in lettuce.  相似文献   

4.
Abstract

In this research the effect of foliar application of selenium (Se) at four levels (Na2OSe4; 0, 5, 10 and 20?mg L?1) was evaluated on some phytochemical characteristics of Sultana grapevine under different salinity levels (NaCl; 0 or 75?mM). The vines were fed twice a week with Hoagland nutrient solution and Se was foliar applied twice with 24 intervals. During growing period, plant height, leaf number and leaf area were recorded. Moreover, at the end of experiment, mature leaves from middle nods of canes were used for measurement of some phytochemical indices. According to results, Se application had a positive effect on plant height, leaf numbers, leaf area and photosynthetic pigments content especially at 5?mg L?1 and to some extent 10?mg L?1 Se levels. Under salinity stress, foliar application of Se at 5?mg L?1 considerably decreased vines leaves electrolyte leakage and lipid peroxidation values compared to non se-treated plants under salinity stress condition. Selenium had an additive effect on salinity stress (75?mM NaCl) induced accumulation of total phenol, total flavonoid, soluble sugars and proline content in leave of vines. Moreover, the interaction of salinity and Se at 5 and 10?mg L?1 improved leaves antioxidant enzymes activities in Sultana grapevine. Likewise, foliar application of Se improved leaf mineral content in 75?mM NaCl -treated vines. Totally, foliar application of selenium (Se at 5 or 10?mg L?1) increased salt tolerance through improvement in nutritional balance and by enzymatic and non-enzymatic antioxidant capacity in grapevine leaves.  相似文献   

5.
The objective of this work was to evaluate the affects of the application of composted biosolids on the accumulation of heavy metals (Cd, Cu, Ni, Pb and Zn) in lettuce leaves. Pots containing different proportions (0 to 100%) of composted biosolids were used to grow lettuce plants under greenhouse conditions. Dry and fresh weight, leaf area and Cd, Cu, Ni, Pb and Zn uptake were determined after harvest. It was found that the dry and fresh matter productions of the plants were significantly lower in the control treatment. The addition of composted biosolids caused a 20 and 40% increase in biomass accumulation. Cd and Pb concentrations in leaves were below detection limits (0.05 mg kg?1) in all treatments. Zn concentration in leaves increases as compost proportion decreases, ranging from 57.2 to 80.4 mg kg?1. Composted biosolids application increased the Cu and Ni plant concentrations, ranging from 5.1 to 9.8 mg Cu kg?1 and 2.3 to 3.7 mg Ni kg?1. In all treatments the proportions of heavy metals in plants were below the international standards of toxicity. The results allow us to suggest that, in short-term applications, composted biosolids could be used as soil amendment for lettuce production, without toxic effects in the chemical composition of the plant.  相似文献   

6.
Abstract

Limited information on the agronomic performance of polyhalite (K2SO4.MgSO4.2CaSO4.2H2O) motivated us to establish two field trials in Sao Paulo, Brazil. The objective was to evaluate the comparative responses of tomato to muriate of potash (MOP), sulfate of potash, potassium magnesium sulfate, and polyhalite at different graded doses of potassium (K) application supplying varied amount of secondary nutrients. Under very low soil K conditions, polyhalite resulted in significantly higher marketable fruit yield, and higher foliar and fruit K and sulfur (S) concentrations than other K sources. This was not the case under medium soil K levels, that is, 101?mg?kg?1. Likewise, polyhalite enhanced postharvest residual soil calcium (Ca), magnesium (Mg), and S than other evaluated sources. Depending on soil nutrient status and the cost of polyhalite, tomato farmers of Brazil could consider polyhalite as an option to meet crop K and secondary nutrient requirements.  相似文献   

7.
ABSTRACT

The effectiveness of nitrogen (N)+ zinc (Zn) soil and foliar fertilizer applications on growth, yield, and quality of apple (Malus domestic Borkh ‘Golden Delicious’) fruit was studied in the Zanjan province, Iran. There were eight treatments 1) control (no fertilizer), 2) soil applied N, 3) soil applied Zn, 4) soil applied N+Zn, 5) foliar applied N, 6) foliar applied Zn, 7) foliar applied N+Zn and 8) combined soil and foliar applied N+Zn. The N source was urea [CO(NH2)2, 46% N] applied at 276 N tree? 1 yr?1 and the Zn source was zinc sulfate (ZnSO4,7H20, 23% Zn) applied at 110 g Zn tree? 1 yr? 1. The soil treatments of N and Zn, were applied every two weeks during June through August (total of 6 times/year) in a 1 m radius around the tree trunk (drip line of trees). The foliar solutions of N (10 g l? 1 urea) and Zn [8 g l? 1 zinc sulfate (ZnSO4)] were sprayed at the rate of 10 L tree? 1 every two weeks at the same times as described for soil applications. The highest yield (49 kg tree? 1), and the heaviest fruits (202 g) were obtained in the soil and foliar combination of N+Zn treatment. The lowest yield (35 kg tree? 1), and the smallest fruits (175 g) were recorded in the control. Nitrogen, and to a lesser extent Zn, foliar application resulted in decreasing fruit quality (caused russeting, and lower soluble solid), but increasing N leaf and fruit concentrations (2.4% DW and 563 mg kg? 1, respectively). There were significant differences among yield and leaf mineral nutrient concentration in different treatments. But there was no significant difference between fruit mineral nutrient concentration (except N). Ratio of N/calcium (Ca), potassium (K)/Ca, and [magnesium (Mg)+K]/Ca in fruits were found suitable for fruit quality prediction. Combining the zinc sulfate with urea in the foliar applications increased the concentration of Zn from 0.7 to 1.5 mg per kg of apple tissue. Leaf N concentration varied during growth season. Foliar applied nutrient can be more efficient than soil applied, but a combination of soil and foliar applications is recommended for apple tree nutrient management.  相似文献   

8.
A pot culture experiment was conducted to study the effect of zinc (Zn) on biofortification of 10 wheat (Triticum aestivum L.) varieties in the Zn-deficient soil of Lucknow. Treatments consisted of 0 and 20 mg Zn kg?1 as a basal dose and 20 mg Zn kg?1 basal dose with two foliar sprays of zinc sulfate (ZnSO4) 0.5%. Foliar sprays of Zn were applied twice at the preflowering stage and 7 days after flowering. Results from the present study revealed that poor growth of plants grown in soil without Zn applications (0 mg Zn kg?1) were improved by applications of Zn (20 mg Zn kg?1) more when Zn was applied with two foliar sprays. Application of Zn (20 mg Zn kg?1) with two foliar sprays also proved beneficial for maximizing Zn concentrations of grains and other plant parts. Wheat varieties NW 1076, K 3827, NW 2036, and UP 262 appeared highly responsive to the treatments.  相似文献   

9.
Runoff and atmospheric chemistry in the Krusne hory Mts. have changed significantly from 1978 to 1994. Forest die-back related deforestation resulted in decreased dry deposition of SO2 and changes in streamwater chemical composition. Atmospheric sulphur (S) deposition decreased from extremely high values of 66.6 kg S ha?1 year?1, in the early 1980s to 35.5 kg S ha?1 year?1 in 1994. Decreasing S input is reflected in decrease of streamwater sulphate (SO4 2?) concentrations, which decreased from 1560 μeq l?1 to 1164 μeq l?1. Runoff export of S was 53 kg S ha?1 year?1 in 1993, S is not retained in the catchments. Nitrogen (N) budget indicates accumulation in the catchment, which is attributed to forest regrowth.  相似文献   

10.
A model deciduous forest soil (Schaffenaker loamy sand) was treated for 8 mo in the greenhouse in 25 cm reconstructed columns with simulated throughfall at pH 6.0 or 4.0, and SO4 2? levels of 12.8 or 24.8 mg L?1. Red oak seedlings grown in the microcosms showed no growth or foliar element response to the treatments. Sulfate loading had a greater impact on soil and leachate chemistry than pH. Higher available soil P in the A, horizon was associated with the pH 6.0 and high SO4 2?2 treatment combination. High SO4 2? loading also reduced exchangeable K+ in the A1?. Other soil horizons were unaffected by either treatment. Leachate chemistry was not significantly altered by througfall pH, but significantly greater export of Na+, Ca2+, Mg2+, Al3+, and NO3 ?, and lower SO4 2? loss, occurred with low SO4 ? input. Comparatively half as much NO3 ? loss was associated with high SO4 2? deposition. The high rate of NO3 ? leaching appeared responsible for greater equivalent mass loss of cations from the low SO4 2? treatment. Leachate removal of SO4 2? approximated input after 8 mo. The capacity of this soil to adsorb SO4 2? appeared relatively limited in the absence of normal element cycling. The sulfate component of simulated deciduous forest throughfall was shown to have a potentially greater impact than pH on ion leaching from forest soil. Additional consideration of the role of SO2? 4 deposition, in the context of throughfall rather than incident precipitation, is warranted in studies of acidic deposition effects on internal forest soil processes.  相似文献   

11.
In 2006–2007 small radish was cultivated in a pot experiment. Foliar applications were applied twice with solutions of the following compounds: 1) control (water); 2) urea; 3) urea+molybdenum (Mo), 4) urea+Mo+benzyladenine (BA); 5) urea+Mo+BA+sucrose; 6) urea+Mo+BA+sucrose+salicylic acid (SA), 7) BA; 8) SA; and 9) sucrose. The above solutions contained following concentrations of compounds: urea 20 g dm?3, sucrose 10 g dm?3, Mo 1 mg dm?3, BA 5 mg dm?3 and SA 10 mg dm?3. In comparison with the control, spraying plants with the solution of urea+Mo+BA+sucrose and SA only caused an increase in leaf mass of one plant. Foliar applications did not have any effect on the yield of edible roots. When compared with the control, the use of sucrose resulted in a decreased content of nitrate (V) in leaves, while the application of urea+Mo+BA+sucrose led to elevated content of nitrate (V) in roots. In case of spraying plants with solutions containing urea (combinations no. 2–6) there was a tendency to increase ammonium (NH4 +) and nitrogen (N)-total content in leaves and roots, and increase in N uptake by leaves and by the whole plant but not by the radish roots. In combinations 7–9 we noted a decline in the level of ascorbic acid, and in combinations 2–6 there was a decrease in the content of soluble sugars in roots. In comparison with the control, an increase was observed in combinations 2 and 3, while in combinations 7–9 a decrease in the content of free amino acids in roots was observed. None of the combinations with foliar application caused any significant changes in the content of assimilative pigments in radish leaves and concentration of nitrate (III), dry matter in leaves and roots, the content of phenolic compounds, content of potassium (K), magnesium (Mg), calcium (Ca) extracted with 2% acetic acid in roots as well as free radical activity of radish roots.  相似文献   

12.
When investigating the reversibility of soil and water acidification due to a reduction of SO42? deposition, the size and stability of the reversibly bound SO42? fraction in soils are important parameters. The desorption behaviour of SO42? in three acid forest soils was investigated using columns with undisturbed and disturbed (< 5 mm sieved) soil material. The results were compared to batch experiments. A comparison of the undisturbed and the disturbed soil samples showed that the soil structure had no effect on the chemistry of the soil solution, the S-mineralisation rates or the SO42? desorption rates. A comparison of the batch and the column method showed only minor differences in desorption rates. However, fitting the measured desorption rates to a modified Langmuir equation showed a more distinct difference between both methods. It was concluded that the batch method was more suitable to establish SO42? desorption isotherms. When investigating SO42? dynamics of soils, the heterogeneity of the soils has to be considered because the spatial variability of isotherm parameters was found to be greater than differences between the investigated methods. Furthermore, SO42? sorption showed a distinct hysteresis. While most of the sorbed SO42? was desorbed at concentrations < 5–10 mg SO42 ?1?1, a sorption of SO42? was observed only at concentrations > 20–30 mg SO42? ·1?1.  相似文献   

13.
ABSTRACT

The volatilization of ammonia is the main reaction that decreases the efficiency of nitrogen fertilization and in order to reduce losses. new technologies such as addition of N-n-butyltriamide thiophosphate (NBPT) to the conventional urea granule (UNBPT) or the covering with polymer and sulfur (UPS) have been developed with the aim to optimize nitrogen fertilization. This work aimed to evaluate the volatilization of ammonia (NH3) in conventional urea (CU) and fertilizers with associated technology under: (a) three temperature conditions (b) and three soil moisture management. The fertilizer CU presented the highest losses by volatilization of 25.93 mg dm?3 while fertilizers with associated technology registered 23.93 mg dm?3 and 8.26 mg dm?3 for UNBPT and UPS. respectively. The highest volatilization of NH3 was registered at 45°C for all fertilizers. Fertilizers with associated technology extended the N-release time. delaying the volatilization peak up to the 6th day or even promoted the gradual release of fertilizer in the soil. such as UPS. The UNBPT showed the lowest volatilization values in the 1st water application. while the CU had lower volatilization values at 25°C (14.48 mg dm?3 NH3) and 35°C (16.99 mg dm?3 NH3) when the matric potential was increased from ?100 to ?50 kPa in the 1st application of water. The UPS did not differ from the volatilization values for the three times of water application.  相似文献   

14.
Abstract

Nitrite (NO2 ?‐N) toxicity symptoms have been observed on lettuce (Lactuca sativa) at various locations in California. The objective was to evaluate the symptoms of ammonium (NH4 +‐N) and nitrite (NO2 ?‐N) toxicity on Sundevil iceberg lettuce and Paragon romaine lettuce and to determine lettuce growth and biomass production under different levels of NO2 ?‐N. Hydroponic studies under greenhouse conditions were conducted using nutrient solutions containing nitrate (NO3 ?‐N) and two other forms of nitrogen (NO2 ?‐N and NH4 +‐N) applied at a constant concentration (50 mg NL?1) or using different NO2 ?‐N levels (0, 5, 10, 20, 30, and 40 mg N L?1) and a constant NO3 ?‐N level (30 mg N L?1). Crown discoloration (brownish color) was observed for lettuce grown in both NO2 ?‐N and NH4 +‐N solutions approximately 3 weeks after transplanting into the hydroponic systems. Lettuce grown in NO3 ?‐N solution produced larger biomass and greater number of leaves per plant than lettuce grown in NO2 ?‐N or NH4 +‐N solutions. Increasing the concentration of NO2 ?‐N suppressed plant height, fresh and dry biomass yield, and number of leaves and increased the root vascular discoloration. Lettuce growth was reduced more than 50% at NO2 ?‐N concentrations greater than 30 mg N L?1. Even at 5 mg NO2 ?‐N L?1, growth was reduced 14 and 24% for romaine and iceberg lettuce, respectively, relative to that obtained in nitrate solution. Although concentrations between 5 and 40 mg NO2 ?‐N L ?1 reduced dry biomass similarly for both lettuce types, toxicity symptoms were more severe in iceberg lettuce than in romaine.  相似文献   

15.
This study evaluated how zinc (Zn) concentration of rice (Oryza sativa L.) seed may be increased and subsequent seedling growth improved by foliar Zn application. Eight foliar Zn treatments of 0.5% zinc sulfate (ZnSO4?·?7H2O) were applied to the rice plant at different growth stages. The resulting seeds were germinated to evaluate effects of seed Zn on seedling growth. Foliar Zn increased paddy Zn concentration only when applied after flowering, with larger increases when applications were repeated. The largest increases of up to ten-fold were in the husk, and smaller increases in brown rice Zn. In the first few days of germination, seedlings from seeds with 42 to 67?mg Zn?kg?1 had longer roots and coleoptiles than those from seeds with 18?mg Zn?kg?1, but this effect disappeared later. The benefit of high seed Zn in seedling growth is also indicated by a positive correlation between Zn concentration in germinating seeds and the combined roots and shoot dry weight (r?=?0.55, p?相似文献   

16.
This study determined the potential to increase Zn density of lettuce (Lactuca sativa L.) through cultivar selection and nutrient management. Organic fertilizer and Hoagland and Arnon no.1 solution factored with three zinc (Zn) levels provided as zinc sulfate (ZnSO4) were the fertilizer regimes in a greenhouse experiment. Modern cultivars had a 32% higher fresh head weight than heritage cultivars, but each accumulated the same Zn concentration (65 mg kg?1 dry wt). Butterhead phenotypes had a 38% lower yield than loose-leaf and had the highest Zn concentration (78 mg kg?1 dry wt) followed by romaine (66 mg kg?1 dry wt) and loose-leaf (53 mg kg?1 dry wt). Concentration of Zn did not differ between fertility regimes, being about 66 mg kg?1 dry wt with each regime. Differences in Zn concentrations were significant among individual cultivars with ranges from 42 mg g?1 dry wt to 91 mg kg?1 dry wt. ‘Tom Thumb’, ‘Adriana’, ‘Claremont’, and ‘Focea’ were the top in cultivar ranking, with mean Zn concentration of 63 mg kg?1 dry wt. The results signify that selection of cultivars may be utilized to increase Zn accumulation in lettuce but that nutritional regimes had little effect on accumulation.  相似文献   

17.
ABSTRACT

Humic (HA) and fulvic (FA) acids improve the nutrient availability and uptake by plants but some aspects of their agronomic use still need to be clarified. The effects of HA soil application and FA foliar application on the growth, Zn and B uptake by coffee seedlings were evaluated. HA was added to an Oxisol at concentrations 0, 10, 25, 50, 75 and 100 mg kg?1 (C-HA), in both limed (pH 6.2) and overlimed (pH 7.2) conditions. FA (0, 0.2, 0.5 and 1 g L?1 C-FA) was applied to coffee leaves in three different application modes (M): with 0.3% Zn and 0.6% B supplied via foliar (M1), 0.6% B and 1.2% Zn supplied via foliar (M2) and 1.2 mg kg?1 B and 6 mg kg?1 Zn supplied via soil (M3). HA addition in soil significantly (p < 0.05) reduced leaf B and Zn accumulation and coffee growth in both pH conditions. In the M1 and M2, FA application significantly (p < 0.05) increased the shoot growth at 0.59 and 0.45 g L?1 and B accumulation at 0.96 and 0.45 g L?1 C-FA. Foliar application of C-FA, instead soil application of C-HA, is a suitable practice to improve coffee seedlings growth and nutrition on Oxisol.  相似文献   

18.
Abstract

Leaching of nutrients and major ions from a tile-drained arable field was evaluated over a 25-year period (1980–2005). The soil, classified as a Gleyic Cambisol, received moderate applications of fertilizers. During later years the soil was more frequently under ley, and since 2002, an area of ravine (29% of the total field) has been managed as a permanent fallow with annual cutting without removing the grass material. A decrease in the concentration of nitrate nitrogen (NO3?N) in the drainwater was estimated in 1980–2005, based on non-parametric tests on concentrations flow-normalized with a robust fitting curve procedure. The average concentration of soluble reactive phosphorus after pre-filtration (RPf) of 0.030 mg l?l corresponded to a calculated degree of phosphorus saturation (DPS) of 6% in acid extract of ammonium lactate from the topsoil. Between 1995 and 2005, concentrations of suspended solids (SS), RP and total organic carbon (TOC) decreased significantly in the drainage water from the entire field. Throughout the entire period, there was a negative net accumulation of the major ions to the soil. The order of decrease in relative terms was calcium (Ca2+)>magnesium (Mg2+)>sulphate (SO4 2?)>chloride (Cl?)>potassium (K+). In addition, the soil phosphorus (P) balance was negative. A significant reduction in ion concentrations in the drainwater, including sodium (Na+) and hydrogen carbonate HCO3 ?, was estimated. The order of reduction in relative terms was: SO4 2?>Mg2+>Ca2+>HCO3 ?>Cl?>NO3 ?>Na+>HPO4. Altogether these trends were equal to approximately 0.1 mmolc l?1. yr?1 of positively and negatively charged ions. Based on measured concentrations, decreasing trends in SO4 2? and Ca2+ were also observed in the shallow groundwater (3.6 m below the soil surface), while K+, Na+ and HCO3 ? tended to increase. Trends of cations in deeper groundwater (5.8 m below the soil surface) were in some cases the opposite of the trends in the drainwater.  相似文献   

19.
《Journal of plant nutrition》2013,36(4-5):613-622
The effectiveness on controlling Fe chlorosis in orange trees grown on calcareous soils was tested. The treatments were Fe(II) sulfate (500 mg Fe L?1), sulfuric acid (0.5 mM H2SO4), Fe(III)-chelate (Hampiron 654 GS, 120 mg Fe L?1) and distilled water as a control. A non-ionic wetting agent was used in all treatments. The use of frequent foliar sprays alleviated Fe chlorosis in orange trees. Sprays of Fe(II) sulfate increased the concentrations of chlorophyll, Fe and zinc in leaves and improved fruit size and quality compared to fruits of control trees. Sprays of Fe(III)-chelate also increased leaf chlorophyll and Fe concentrations and improved fruit quality, but did not increase fruit size. Sprays of sulfuric acid alone slightly increased leaf chlorophyll and Fe concentrations, without improving fruit size and quality. These results suggest that foliar sprays with Fe could help to avoid yield and quality losses caused by Fe chlorosis in citrus orchards. Furthermore, these treatments could be done with relatively cheap materials such as solutions containing Fe(II) sulfate.  相似文献   

20.
Sulfate (SO4 2?), nitrate (NO3 ?) and ammonium (NH4 +) concentrations in precipitation as measured at NADP sites within the Ohio River Valley of the Midwestern USA between 1985 and 2002 are quantified and temporal trends attributed to changes/ variations in (i) the precipitation regime, (ii) emission patterns and (iii) air mass trajectories. The results indicate that mean SO4 2? concentrations in precipitation declined by 37–43% between 1985 and 2002, while NO3 ? concentrations decreased by 1–32%, and NH4 + concentrations exhibited declining concentrations at some sites and increasing concentrations at others. The change in SO4 2? concentrations is in broad agreement with estimated reductions in sulfur dioxide emissions. Changes in NO3 ? concentrations appear to be less closely related to variations in emissions of oxides of nitrogen and exhibit a stronger dependence on weekly precipitation volume. Up to one quarter of the variability in log-transformed weekly NO3 ? concentrations in precipitation is explicable by variations in precipitation volume. Trends in annual average log-transformed SO4 2? concentrations exhibit only a relatively small influence of variability in weekly precipitation amount but at each of the sites considered the variance explanation of annual average log-transformed SO4 2? by sampling year was increased by removing the influence of precipitation volume. Annual mean log-transformed ion concentrations detrended for precipitation volume (by week) and emission changes (by year) exhibit positive correlations at all sites, indicating that the residual variability of SO4 2?, NO3 ? and NH4 + may have a common source which is postulated to be linked to synoptic scale variability and air mass trajectories.  相似文献   

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