Nitro-PAHs and PAHs in Atmospheric Particulate Matters and Sea Sediments in Hiroshima Bay Area, Japan |
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| Authors: | Noriatsu Ozaki Nobuya Takemoto Tomonori Kindaichi |
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| Institution: | 1. Graduate School of Engineering, Hiroshima University, 1-4-1 Kagamiyama, Higashihiroshima, 739-8527, Hiroshima, Japan
2. Okayama Prefectural Bureau, 2-4-6 Uchiyamashita, Okayama, 700-8570, Okayama, Japan
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| Abstract: | Atmospheric and sea sediment concentrations were measured for eight nitrated polycyclic aromatic hydrocarbons (nitro-PAHs) and three unsubstituted PAHs in a suburban area and sea sediments in the Hiroshima Bay watershed area, Japan, from July to December, 2006 (atmospheric particulate matter) and in September and November, 2004 (sea sediments). Atmospheric concentration was higher in winter than summer for both nitro-PAHs and PAHs. Concentrations in sea sediments were less than 10%, and pattern was similar to those of atmospheric particles. Several combustion emission sources were also measured, and the 1-NP/Pyr ratio was compared to environmental values. The ratio of atmospheric and sea sediments were significantly lower than diesel particulate matters. Further, the vehicle emission loading and sea sedimentation loading was evaluated in this watershed area, and from the comparison, the existence of other important sources PAHs were suggested. |
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