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地质封存CO2泄露对地表水中非金属类指标的影响
引用本文:张丙华,景炯炯,耿春香,张倩.地质封存CO2泄露对地表水中非金属类指标的影响[J].水土保持通报,2016,36(2):161-164,170.
作者姓名:张丙华  景炯炯  耿春香  张倩
作者单位:1. 中国石油大学(华东)理学院,山东青岛,266580;2. 中国石油大学(华东)化学工程学院,山东青岛,266580
摘    要:目的]探讨地质封存CO_2泄露对地表水中非金属类物质指标的影响,为相关研究提供理论依据。方法]通过控制二氧化碳泄露时间、泄露速率、泄漏时的温度等条件,分析其对地表水中pH值、溶解氧(DO)、HCO-3和化学需氧量(COD)等指标的影响。结果]一定时间内,二氧化碳泄露对pH值和DO的影响最大,对HCO-3和COD的影响较小;泄露速率的增大将提高pH,DO,HCO-3的反应速率,即加快pH值和DO的下降,加快了HCO-3的升高;而温度的升高对COD的影响最大。结论]建议将地质封存CO_2的监测指标选取为地表水中的pH值、DO和HCO-3,因为此三者的变化明显。

关 键 词:环境  碳捕捉与封存技术  二氧化碳泄露  地表水  非金属类指标
收稿时间:2015/10/22 0:00:00
修稿时间:2015/11/19 0:00:00

Influence on Non-metallic Parameters of Surface Water for Leakage of Carbon Dioxide During Geological Storage
ZHANG Binghu,JING Jiongjiong,GENG Chunxiang and ZHANG Qian.Influence on Non-metallic Parameters of Surface Water for Leakage of Carbon Dioxide During Geological Storage[J].Bulletin of Soil and Water Conservation,2016,36(2):161-164,170.
Authors:ZHANG Binghu  JING Jiongjiong  GENG Chunxiang and ZHANG Qian
Institution:School of Science, China University of Petroleum(East China), Qingdao, Shandong 266580, China,School of Chemical Engineering, China University of Petroleum(East China), Qingdao, Shandong 266580, China,School of Chemical Engineering, China University of Petroleum(East China), Qingdao, Shandong 266580, China and School of Chemical Engineering, China University of Petroleum(East China), Qingdao, Shandong 266580, China
Abstract:Objective] Studying the effect of CO2 leakage during geological storage on non-metallic surface water in order to provide a theoretical basis for the related research. Methods] By changing the leakage time, leakage rate, and the temperature of carbon dioxide, we studied the impacts on pH value, DO, HCO3- and COD of surface water. Results] The leakage of CO2 affected pH and DO value greatly, whereas its effects on HCO3- and COD were relatively small. Increasing of leakage rate could accelerate the reaction rate of pH, DO and HCO3-, thereby pH and DO declined faster, and HCO3- increased more quickly. However, temperature rising had the greatest impact on COD content. Conclusion] It suggests that pH, DO and HCO3-, as their sensitive reaction to CO2, could be used as the surface water monitoring indicators for CO2 geological storage.
Keywords:environment  carbon capture and storage  CO2 leakage  surface water  non-metallic parameters
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